Mixed-mode oscillations in a homogeneous pH-oscillatory chemical reaction system

We examine experimentally a chemical system in a flow-through stirred reactor, which is known to provide large-amplitude oscillations of the pH value. By systematic variation of the flow rate, we find that the system displays hysteresis between a steady state and oscillations, and more interestingly, a transition to chaos involving mixed-mode oscillations. The basic pattern of the measured pH in the mixed-mode regime includes a large-scale peak followed by a series of oscillations on a much smaller scale, which are usually highly irregular and of variable duration. The bifurcation diagram shows that chaos sets in via a period-doubling route observed on the large-amplitude scale, but simultaneously small-amplitude oscillations are involved. Beyond the apparent accumulation of period doubling bifurcations, a mixed-mode regime with irregular oscillations on both scales is observed, occasionally interrupted by windows of periodicity. As the flow rate is further increased, chaos turns into quasiperiodicity and later to a simple small-amplitude periodic regime. Dynamics of selected typical regimes were examined with the tools of nonlinear time-series analysis, which include phase space reconstruction of an attractor and calculation of the maximal Lyapunov exponent. The analysis points to deterministic chaos, which appears via a period doubling route from below and via a route involving quasiperiodicity from above, when the flow rate is varied.     

Oscillations, period doublings, and chaos in CO oxidation and catalytic mufflers

Early experimental observations of chaotic behavior arising via the period-doubling route for the CO catalytic oxidation both on Pt(110) and Ptgamma-Al(2)O(3) porous catalyst were reported more than 15 years ago. Recently, a detailed kinetic reaction scheme including over 20 reaction steps was proposed for the catalytic CO oxidation, NO(x) reduction, and hydrocarbon oxidation taking place in a three-way catalyst (TWC) converter, the most common reactor for detoxification of automobile exhaust gases. This reactor is typically operated with periodic variation of inlet oxygen concentration. For an unforced lumped model, we report results of the stoichiometric network analysis of a CO reaction subnetwork determining feedback loops, which cause the oscillations within certain regions of parameters in bifurcation diagrams constructed by numerical continuation techniques. For a forced system, numerical simulations of the CO oxidation reveal the existence of a period-doubling route to chaos. The dependence of the rotation number on the amplitude and period of forcing shows a typical bifurcation structure of Arnold tongues ordered according to Farey sequences, and positive Lyapunov exponents for sufficiently large forcing amplitudes indicate the presence of chaotic dynamics. Multiple periodic and aperiodic time courses of outlet concentrations were also found in simulations using the lumped model with the full TWC kinetics. Numerical solutions of the distributed model in two geometric coordinates with the CO oxidation subnetwork consisting of several tens of nonlinear partial differential equations show oscillations of the outlet reactor concentrations and, in the presence of forcing, multiple periodic and aperiodic oscillations. Spatiotemporal concentration patterns illustrate the complexity of processes within the reactor.     

Feedback control of canards

We present a control mechanism for tuning a fast-slow dynamical system undergoing a supercritical Hopf bifurcation to be in the canard regime, the tiny parameter window between small and large periodic behavior. Our control strategy uses continuous feedback control via a slow control variable to cause the system to drift on average toward canard orbits. We apply this to tune the FitzHugh-Nagumo model to produce maximal canard orbits. When the controller is improperly configured, periodic or chaotic mixed-mode oscillations are found. We also investigate the effects of noise on this control mechanism. Finally, we demonstrate that a sensor tuned in this way to operate near the canard regime can detect tiny changes in system parameters.     

一个简单延迟非线性系统的动力学行为及混沌同步

分析一个简单二阶延迟系统的Hopf分支和混沌特性, 包括分支点、分支方向和分支周期解的稳定性, 解析求出退延迟情况下, 这个系统的相轨线方程; 通过数值计算并绘制分岔图, 揭示系统存在由倍周期通向混沌的道路; 利用单路线性组合信号, 反馈控制实现系统的部分完全同步; 利用主动-被动与线性反馈的联合, 实现系统的完全同步; 设计和搭建系统的电子实验线路, 并从实验中观测到与理论分析或数值计算相一致的结果. 关键词： 延迟非线性系统 电路实验 Hopf分支 混沌     

Multimode semiconductor laser with selective optical feedback

We study a multimode semiconductor laser subject to moderate selective optical feedback. The steady state of the laser is destabilized by a Hopf bifurcation and exhibits a period-doubling route to chaos. We also show the existence of a heteroclinic connection between a saddle node and an unstable focus that can be associated with experimentally observed multimode low-frequency fluctuations. This heteroclinic connection coexists with a chaotic attractor resulting from the period-doubling process.     

Period-doubling cascades of canards from the extended Bonhoeffer-van der Pol oscillator

This Letter investigates the period-doubling cascades of canards, generated in the extended Bonhoeffer-van der Pol oscillator. Canards appear by Andronov-Hopf bifurcations (AHBs) and it is confirmed that these AHBs are always supercritical in our system. The cascades of period-doubling bifurcation are followed by mixed-mode oscillations. The detailed two-parameter bifurcation diagrams are derived, and it is clarified that the period-doubling bifurcations arise from a narrow parameter value range at which the original canard in the non-extended equation is observed.     

Dynamics of erbium-doped fibre laser with optical delay feedback and chaotic synchronization

The dynamical behaviour of the erbium-doped fibre single-ring laser with an optical delay feedback is discussed. Simulation shows that as the delay rate increases, the lasing light displays period-doubling which leads to chaos and via reverse period-doubling route returns from chaos to periodic. At a particular delay rate the intermittently chaotic route to chaos is also observed. The identical synchronization based on chaos in this ring laser is demonstrated by numerical simulation.     

线性延时反馈Josephson结的Hopf分岔和混沌化

考虑线性延时反馈控制下电阻-电容分路的Josephson结,运用非线性动力学理论分析了受控系统平凡解的稳定性.理论分析表明,随着控制参数的改变,系统的稳定平凡解将会通过Hopf分岔失稳,并推导了发生Hopf分岔的临界参数条件.对不同参数条件下受控系统的动力学进行了数值分析.结果显示,系统由Hopf分岔产生的稳定周期解,将进一步通过对称破缺分岔和倍周期分岔通向混沌. 关键词： 约瑟夫森结 线性延时反馈 Hopf分岔 混沌     

Nonlinear oscillations and chaotic behavior due to impact lonization of shallow donors in InSb

Both nonlinear oscillations and chaotic behavior in n-InSb are experimentally investigated for the case of impact ionization of shallow donors at low temperatures. Complex behavior including a simple periodic oscillation, a period-doubling route to chaos, and quasiperiodic behavior are observed with increasing electric field as the parameter. For the first time, a type of pitchfork bifurcation (period halving) is seen.     

Theory of stability and bifurcation in a multi-quantum well laser with opto-electronic delayed feedback

This paper presents an opto-electronic feedback multi-quantum well laser system and outlines our study of the dynamics and bifurcation in a multi-quantum well laser due to the opto-electronic delayed feedback effect. We point out theoretically the conditions of stability and Hopf bifurcation of the laser. The relaxation oscillation frequency of the system is educed to be the function of the feedback level, delayed time and in-current. The route from stability to bifurcation is numerically simulated via varying the delayed time, feedback strength and in-current. The results show that the induced dynamics can be grouped into four distinct types or modes (stable, periodic pulsed, undamped oscillating or beating, and chaos), where the frequency and intensity varying with the delayed time in the two periodic regions are analyzed detailedly to find that the pulsing frequency is reduced with the long delayed time while the pulsing intensity is added with the long delayed time. And the chaotic pulsing frequency is increased with the large in-current. In addition, the carrier transport between the barrier region and the active region can characterize the dynamics in the laser to produce stable, periodic pulsed, beating and chaotic states by altering the carriers transport or escape rate value.     

Multiple period-doubling bifurcation route to chaos in periodically pulsed Murali-Lakshmanan-Chua circuit-controlling and synchronization of chaos

We consider a simple nonautonomous dissipative nonlinear electronic circuit consisting of Chua's diode as the only nonlinear element, which exhibit a typical period doubling bifurcation route to chaotic oscillations. In this paper, we show that the effect of additional periodic pulses in this Murali-Lakshmanan-Chua (MLC) circuit results in novel multiple-period-doubling bifurcation behavior, prior to the onset of chaos, by using both numerical and some experimental simulations. In the chaotic regime, this circuit exhibits a rich variety of dynamical behavior including enlarged periodic windows, attractor crises, distinctly modified bifurcation structures, and so on. For certain types of periodic pulses, this circuit also admits transcritical bifurcations preceding the onset of multiple-period-doubling bifurcations. We have characterized our numerical simulation results by using Lyapunov exponents, correlation dimension, and power spectrum, which are found to be in good agreement with the experimental observations. Further controlling and synchronization of chaos in this periodically pulsed MLC circuit have been achieved by using suitable methods. We have also shown that the chaotic attractor becomes more complicated and their corresponding return maps are no longer simple for large n-periodic pulses. The above study also indicates that one can generate any desired n-period-doubling bifurcation behavior by applying n-periodic pulses to a chaotic system.     

Dynamics and stabilization of peak current-mode controlled buck converter with constant current load

The discrete iterative map model of peak current-mode controlled buck converter with constant current load(CCL),containing the output voltage feedback and ramp compensation, is established in this paper. Based on this model the complex dynamics of this converter is investigated by analyzing bifurcation diagrams and the Lyapunov exponent spectrum. The effects of ramp compensation and output voltage feedback on the stability of the converter are investigated. Experimental results verify the simulation and theoretical analysis. The stability boundary and chaos boundary are obtained under the theoretical conditions of period-doubling bifurcation and border collision. It is found that there are four operation regions in the peak current-mode controlled buck converter with CCL due to period-doubling bifurcation and border-collision bifurcation. Research results indicate that ramp compensation can extend the stable operation range and transfer the operating mode, and output voltage feedback can eventually eliminate the coexisting fast-slow scale instability.     

Mixed-mode oscillations in a stochastic,piecewise-linear system

We analyse a piecewise-linear FitzHugh–Nagumo model. The system exhibits a canard near which both small amplitude and large amplitude periodic orbits exist. The addition of small noise induces mixed-mode oscillations (MMOs) in the vicinity of the canard point. We determine the effect of each model parameter on the stochastically driven MMOs. In particular we show that any parameter variation (such as a modification of the piecewise-linear function in the model) that leaves the ratio of noise amplitude to time-scale separation unchanged typically has little effect on the width of the interval of the primary bifurcation parameter over which MMOs occur. In that sense, the MMOs are robust. Furthermore, we show that the piecewise-linear model exhibits MMOs more readily than the classical FitzHugh–Nagumo model for which a cubic polynomial is the only nonlinearity. By studying a piecewise-linear model, we are able to explain results using analytical expressions and compare these with numerical investigations.     

Dynamic characteristics in an external-cavity multi-quantum-well laser

This paper outlines our studies of bifurcation, quasi-periodic road to chaos and other dynamic characteristics in an external-cavity multi-quantum-well laser with delay optical feedback. The bistable state of the laser is predicted by finding theoretically that the gain shifts abruptly between two values due to the feedback. We make a linear stability analysis of the dynamic behavior of the laser. We predict the stability scenario by using the characteristic equation while we make an approximate analysis of the stability of the equilibrium point and discuss the quantitative criteria of bifurcation. We deduce a formula for the relaxation oscillation frequency and prove theoretically that this formula function relates to the loss of carriers transferring between well regime and barrier regime, the feedback level, the delayed time and the other intrinsic parameters. We demonstrate the dynamic distribution and double relaxation oscillation frequency abruptly changing in periodic states and find the multi-frequency characteristic in a chaotic state. We illustrate a road to chaos from a stable state to quasi-periodic states by increasing the feedback level. The effects of the transfers of carriers and the escaping of carriers on dynamic behavior are analyzed, showing that they are contrary to each other via the bifurcation diagram. Also,we show another road to chaos after bifurcation through changing the linewidth enhancement factor, the photon loss rate and the transfer rate of carriers.     

Deterministic chaos in a diode-pumped Nd:YAG laser passively Q switched by a Cr4+:YAG crystal

We report the experimental observation and numerical simulation of deterministic chaos in a diode-pumped Nd:YAG solid-state laser that is passively Q switched by a Cr4+:YAG crystal saturable absorber. We show that apart from the stable Q-switched operation the laser can also exhibit complicated nonlinear dynamics, including the period-doubling route to chaos and periodic windows.     

Dynamical behaviors of a chaotic system with no equilibria

Based on Sprott D system, a simple three-dimensional autonomous system with no equilibria is reported. The remarkable particularity of the system is that there exists a constant controller, which can adjust the type of chaotic attractors. It is demonstrated to be chaotic in the sense of having a positive largest Lyapunov exponent and fractional dimension. To further understand the complex dynamics of the system, some basic properties such as Lyapunov exponents, bifurcation diagram, Poincaré mapping and period-doubling route to chaos are analyzed with careful numerical simulations.     

Fluctuations and simple chaotic dynamics

We describe the effects of fluctuations on the period-doubling bifurcation to chaos. We study the dynamics of maps of the interval in the absence of noise and numerically verify the scaling behavior of the Lyapunov characteristic exponent near the transition to chaos. As previously shown, fluctuations produce a gap in the period-doubling bifurcation sequence. We show that this implies a scaling behavior for the chaotic threshold and determine the associated critical exponent. By considering fluctuations as a disordering field on the deterministic dynamics, we obtain scaling relations between various critical exponents relating the effect of noise on the Lyapunov characteristic exponent. A rule is developed to explain the effects of additive noise at fixed parameter value from the deterministic dynamics at nearby parameter values.     

Spiking behavior in a noise-driven system combining oscillatory and excitatory properties

We show that firing activity (spiking) can be regularized by noise in a FitzHugh-Nagumo (FHN) neuron model when operating slightly beyond the supercritical Hopf bifurcation (in the "canard" region). We also provide the conditions for imperfect phase locking between interspike intervals and low amplitude quasiharmonic oscillations. For the imperfect phase locking no need exists of an external signal as it follows from the FHN intrinsic dynamics.     

Nonlinear dynamics and chaos analysis of one-dimensional pulsating detonations

To understand the nonlinear dynamical behaviour of a one-dimensional pulsating detonation, results obtained from numerical simulations of the Euler equations with simple one-step Arrhenius kinetics are analysed using basic nonlinear dynamics and chaos theory. To illustrate the transition pattern from a simple harmonic limit-cycle to a more complex irregular oscillation, a bifurcation diagram is constructed from the computational results. Evidence suggests that the route to higher instability modes may follow closely the Feigenbaum scenario of a period-doubling cascade observed in many generic nonlinear systems. Analysis of the one-dimensional pulsating detonation shows that the Feigenbaum number, defined as the ratio of intervals between successive bifurcations, appears to be in reasonable agreement with the universal value of d = 4.669. Using the concept of the largest Lyapunov exponent, the existence of chaos in a one-dimensional unsteady detonation is demonstrated.     

Wideband chaos generation using a delayed oscillator and a two-dimensional nonlinearity induced by a quadrature phase-shift-keying electro-optic modulator

We present a new optoelectronic architecture intended for chaotic optical intensity generation. The principle relies on an electro-optic nonlinear delay dynamics, where the nonlinearity originates from an integrated four-wave optical interferometer, involving two independent electro-optic modulation inputs. Consequently, the setup involves both two-dimensional nonlinearity and dual-delay feedback dynamics, which results in enhanced chaos complexity of particular interest in chaos encryption schemes. The generated chaos observed with large feedback gains has a bandwidth ranging from 30 kHz to 13 GHz and is confirmed by numerical simulations of the proposed dynamical model and bifurcation diagram calculation.