Frequency stabilization and measurements of 543 nm HeNe lasers

In this paper we report our investigations on the frequency stabilization and frequency measurements of 543 nm HeNe laser. It contains following four different works. (1) Using a metal laser tube we have built an iodine-stabilized 543 nm HeNe laser by the Frequency-Modulation (FM) spectroscopy. The signal-to-noise ratio of the hyperfine spectrum reached 2 × 10^–12 at 1 s sampling time. (2) We have built a compact iodine-stabilized 543 nm HeNe laser system using the third-harmonic locking technique. Stability better than 1 × 10^–12 for sampling time >1 s is obtained. We also suggest the b₁₀ line for the future recommendation. (3) We constructed the Lamb-dip stabilized He-²⁰Ne and He-²²Ne lasers and measured their frequency stability, reproducibility, and absolute frequencies. The results suggest that the Lamb-dip stabilized lasers are appropriate for secondary wavelength standards. We have also deduced the isotope shift of Ne atom at 543 nm. (4) We have developed two two-mode stabilized 543 nm HeNe lasers using the bang-bang control method. The Allan variance is 1 × 10^–11 at 1 s sampling time.     

A diode laser spectrometer at 634nm and absolute frequency measurements using optical frequency comb

This paper reports that two identical external-cavity-diode-laser (ECDL) based spectrometers are constructed at 634 nm referencing on the hyperfine B-X transition R(80)8-4 of ¹²⁷I₂. The lasers are stabilized on the Doppler-free absorption signals using the third-harmonic detection technique. The instability of the stabilized laser is measured to be 2.8×10^-12 (after 1000 s) by counting the beat note between the two lasers. The absolute optical frequency of the transition is, for the first time, determined to be 472851936189.5 kHz by using an optical frequency comb referenced on the microwave caesium atomic clock. The uncertainty of the measurement is less than 4.9 kHz.     

Efficient diode-pumped Nd:YVO4 continuous-wave laser at 1.34 μm

We report a high-power continuous-wave(cw) diode-pumped efficient 1.34 μm Nd:YVO₄ laser. The laser properties of a low Nd³⁺-doped concentration of the Nd:YVO₄ crystal operating at 1.34 μm formed with a simple plane-concave cavity have been demonstrated. With the incident pump power of 22 W, an output power of 8.24 W was obtained, giving an optical conversion efficiency of 37.5% and slope efficiency of 40%. The thermal effects of cw end-pumped solid-state lasers were studied.     

Heterodyne frequency measurements of carbonyl sulfide transitions at 26 and 51 THz. Improved OCS,O13CS,and OC34S molecular constants

Heterodyne frequency measurements were made on selected absorption features of carbonyl sulfide (OCS) near 26 THz (860 cm^?1) and 51 THz (1700 cm^?1). Frequency differences were measured between a tunable diode laser (TDL) locked to carbonyl sulfide absorption lines and either a stabilized ¹³CO₂ laser or a CO laser which was referred to stabilized CO₂ lasers. These measurements are combined with conventional TDL measurements and published microwave measurements to obtain new, more reliable molecular constants for OCS, O¹³CS, and OC³⁴S. New frequency measurements are given for nine CO laser transitions between 1686 and 1726 cm^?1.     

Frequency comb-referenced narrow line width diode laser system for coherent molecular spectroscopy

We analyze in detail the frequency noise properties of a grating enhanced external cavity diode laser (GEECDL). This system merges two diode laser concepts, the grating stabilized diode laser and the diode laser with resonant optical feedback, thus combining a large tuning range with an excellent short-term frequency stability. We compare the frequency noise spectrum of a GEECDL to that of a grating stabilized diode laser and demonstrate a 10-fold reduction of the frequency noise linear spectral density. The GEECDL is phase locked to a similar laser and to a fs-frequency comb with a servo loop providing an open-loop unity-gain frequency of only 237 kHz, which is a tenth of the bandwidth typically required for grating stabilized diode lasers. We achieve a residual rms phase error as small as 72 mrad (≈ 200 mrad) for stabilization to a similar laser (to the fs-frequency comb). We demonstrate that the novel diode laser can phase-coherently track a stable optical reference with an instability of 1.8×10^-16 at 1 s. This laser system is well suited for applications that require phase locking to a low-power optical reference under noisy conditions. It may also be considered for the implementation of optical clock lasers. PACS 42.55.Px; 42.60.Jf; 42.50.Gy     

A broadband ytterbium-doped tunable fiber laser for <Superscript>3</Superscript>He optical pumping at 1083 nm

Large amounts of hyperpolarized ³He gas with high nuclear polarization rates are required for use in neutron spin filters or nuclear magnetic resonance imaging of human lung. Very high efficiency can be obtained by metastability exchange optical pumping using multimode lasers to excite the ^[ 2 _]3S-^[ 2 _]3P transition at 1083 nm. Broadband ytterbium-doped tunable fiber lasers have been designed for that particular application. Different options for the architecture of the fiber oscillator are presented and compared. Emphasis is given to a linear cavity configuration that includes a high reflectivity fiber mirror and a low reflectivity tunable fiber Bragg grating. Optical measurements are performed to finely characterize the spectral behavior of the lasers. Atomic response is also quantitatively probed to assess the optimal design of the oscillator for optical pumping. Multimode operation matching the 2 GHz Doppler-broadened helium resonance line and tunability over more than 200 GHz are demonstrated. Boosting the output of this fiber laser with a Yb-doped fiber power amplifier, all-fiber devices are built to provide robust, high-power turnkey sources at 1083 nm for improved production of laser polarized ³He. PACS 42.60.-v; 42.55.Wd; 32.80.Bx     

Intermittent frequency offset lock of a symmetric three-mode stabilized He-Ne laser to an iodine stabilized He-Ne laser

There is a need for an intense, unmodulated single-frequency stabilized laser light that guarantees absolute optical frequency in a rapid laser calibration or an ultra-high resolution interferometer. To obtain such a light, we developed a new laser system that uses an intermittent frequency offset lock of a symmetric three-mode stabilized He-Ne laser to an iodine stabilized He-Ne laser. The proposed laser system provides two operational modes: (1) independent and (2) slave mode. In the independent mode, frequency of the three-mode laser is stabilized via control of frequency difference between two intermode beats. The resultant output is a single longitudinal mode light of maximum intensity that locates at the top of the gain curve. Frequency instability of 8X10^-12 (at a sampling time of 100 s) which is better than conventional stabilized lasers is attained in the independent mode. Slow optical frequency drift during the independent mode is periodically corrected by the offset lock to the iodine stabilized laser (slave mode), resulting in accurate reset of the frequency drift. After reset of the frequency deviation, the three-mode laser is again operated in the independent mode. Due to such intermittent offset lock, duty factor of the iodine stabilized laser was reduced to a few % of continuous operation.     

Frequency tuning peculiarities of enhanced power monomode He−Ne lasers

Experimental results are presented concerning some peculiarities of frequency tuning of single-longitudinal-mode He–Ne lasers at 632.8 nm which single-mode selection is performed by increasing the homogeneous broadening of laser transition. These include the observation of an asymmetry of tuning regions with respect to the output power maximum; a jump of lasing frequency during which output power drops; and a strong dependence of frequency tuning on gas pressure and output power. In the case of a mixture of ²⁰Ne and ²²Ne isotopes, analytical expressions for the dependence on frequency of output power, unsaturated gain and saturated gain are obtained and computed at different neon isotope concentrations, gas pressures and cavity losses. Simultaneous consideration of these dependences is proposed and used for an explanation of experimentally observed peculiarities in frequency tuning. The obtained results could be used for realization of a frequency-stabilized He–Ne laser of a few milliwatts power for the purposes of multidimensional interferometric measurements.     

Tapered diode lasers and laser modules near 635nm with efficient fiber coupling for flying-spot display applications

Flying-spot displays require light sources in the red, green and blue with a high optical output power and nearly diffraction limited beams. In this paper we present experimental results of red-emitting, AlGaInP based, tapered diode lasers and their integration into diode laser modules. The laser modules emit a collimated, almost diffraction limited beam with an optical output power as high as 1W at a wavelength close to 635 nm. The tapered laser chips were designed with emphasis on achieving a good beam quality in vertical and lateral directions of a collimated beam. To test the suitability for flying-spot display applications, we performed fiber coupling experiments with a low mode number optical fiber with an etendue as low as 6 × 10^?6 mm² sr. A maximum transmission of 70% of the launched power behind the uncoated fiber as well as a usable power in excess of 580mW were measured.     

Locking the frequency of lasers to an optical cavity at the 1.6×10−17 relative instability level

We stabilized the frequencies of two independent Nd:YAG lasers to two adjacent longitudinal modes of a high-finesse Fabry–Pérot resonator and obtained a beat frequency instability of 6.3 mHz at an integration time of 40 s. Referred to a single laser, this is 1.6×10^?17 relative to the laser frequency, and 1.3×10^?6 relative to the full width at half maximum of the cavity resonance. The amplitude spectrum of the beat signal had a FWHM of 7.8 mHz. This stable frequency locking is of importance for next-generation optical clock interrogation lasers and fundamental physics tests.     

A neodymium fluid laser: Laser emission in circulating state

Differing from conventional liquid lasers, a novel concept of fluid laser was provided, which has attractively potential using in high average power lasers. The laser medium was prepared by dispersing Nd³⁺: phosphate glass micro-balls in organic match liquid. Its optical properties were investigated and the radiative transition rate was calculated by Judd–Ofelt theory. The experiment of laser oscillation in static state indicates that the heat exchanging has limited effect on refractive index of the fluid laser medium in a short time. In circulating state, a laser oscillation occurred at 1058.1 nm when pumped by two 808 nm diode lasers. The maximum output energy is 2.58 mJ with the absorbed pumping energy of 460 mJ. This study offers a new way in the exploration of high average power laser.     

Laser frequency stabilization at 1.5 microns using ultranarrow inhomogeneous absorption profiles in Er:LiYF4

Single-frequency diode lasers have been frequency stabilized to 1.5 kHz Allan deviation over 0.05-50 s integration times, with laser frequency drift reduced to less than 1.4 kHz/min, using the frequency reference provided by an ultranarrow inhomogeneously broadened Er³⁺:⁴I_15/2→⁴I_13/2 optical absorption transition at a vacuum wavelength of 1530.40 nm in a low-strain LiYF₄ crystal. The 130 MHz full-width at half-maximum (FWHM) inhomogeneous line width of this reference transition is the narrowest reported for a solid at 1.5 μm. Strain-induced inhomogeneous broadening was reduced by using the single isotope ⁷Li and by the very similar radii of Er³⁺ and the Y³⁺ ions for which it substitutes. To show the practicability of cryogen-free cooling, this laser stability was obtained with the reference crystal at 5 K; moreover, this performance did not require vibrational isolation of either the laser or crystal frequency reference. Stabilization is feasible up to T=25 K where the Er³⁺ absorption thermally broadens to ∼500 MHz. This stabilized laser system provides a tool for interferometry, high-resolution spectroscopy, real-time optical signal processing based on spatial spectral holography and accumulated photon echoes, secondary frequency standards, and other applications such as quantum information science requiring narrow-band light sources or coherent detection.     

Detection of methane in air using diode-laser pumped difference-frequency generation near 3.2 μm

Spectroscopic detection of the methane in natural air using an 800 nm diode laser and a diode-pumped 1064 nm Nd:YAG laser to produce tunable light near 3.2 µm is reported. The lasers were pump sources for ring-cavity-enhanced tunable difference-frequency mixing in AgGaS₂. IR frequency tuning between 3076 and 3183 cm^–1 was performed by crystal rotation and tuning of the extended-cavity diode laser. Feedback stabilization of the IR power reduced intensity noise below the detector noise level. Direct absorption and wavelength-modulation (2f) spectroscopy of the methane in natural air at 10.7 kPa (80 torr) were performed in a 1 m single-pass cell with 1 µW probe power. Methane has also been detected using a 3.2 µm confocal build-up cavity in conjunction with an intracavity absorption cell. The best methane detection limit observed was 12 ppb m (Hz.)^–1/2.     

Diode laser based light sources for biomedical applications

Diode lasers are by far the most efficient lasers currently available. With the ever‐continuing improvement in diode laser technology, this type of laser has become increasingly attractive for a wide range of biomedical applications. Compared to the characteristics of competing laser systems, diode lasers simultaneously offer tunability, high‐power emission and compact size at fairly low cost. Therefore, diode lasers are increasingly preferred in important applications, such as photocoagulation, optical coherence tomography, diffuse optical imaging, fluorescence lifetime imaging, and terahertz imaging. This review provides an overview of the latest development of diode laser technology and systems and their use within selected biomedical applications. 670 nm external cavity diode laser for Raman spectroscopy built on a 13 × 4 mm² microbench (Copyright FBH/Schurian.com ).     

Method to investigate the symmetry of saturated absorption signals by means of laser frequency locking techniques

It is shown that the line shape of a saturated absorption signal — especially its symmetry — can be investigated by combining laser frequency locking methods. The laser frequencyv, modulated with a frequencyf, is stabilized alternatively to the zero crossings of the synchronously detected 2f and 3f absorption signals. In addition, almost any other part of the profile can be tested by locking the laser frequency to neighboruing points of the zero crossings by using an offset technique. With two prestabilized Ar⁺ lasers atv=582 THz the symmetry of different¹²⁷ I ₂ hfs signals was investigated with an uncertainty of typically 2×10^–12 v or 10^–3 halfwidths.     

Concept of neutral gain modules for power scaling of thin-disk lasers

We present a concept for power scaling of high brightness solid state lasers, which introduces so called gain modules containing the laser active media. These modules can be inserted as relay imaging optical systems in any type of laser resonators. The gain modules are optically neutral; hence, power scaling can be provided inserting several modules. Here, we provide the basic functional units of gain modules as well as an exemplary experimental implementation in thin-disk lasers with dynamically stable resonators. On the basis of these studies, more than 1 kW output power with an averaged M ²=2.6 could be demonstrated using two disks. Experiments with four disks are in preparation.     

A three-step laser stabilization scheme for excitation to Rydberg levels in <Superscript>85</Superscript>Rb

We demonstrate a three-step laser stabilization scheme for excitation to nP and nF Rydberg states in ⁸⁵Rb, with all three lasers stabilized using active feedback to independent Rb vapor cells. The setup allows stabilization to the Rydberg states 36P_3/2–70P_3/2 and 33F_7/2–90F_7/2, with the only limiting factor being the available third step laser power. We study the scheme by monitoring the three laser frequencies simultaneously against a self-referenced optical frequency comb. The third step laser, locked to the Rydberg transition, displays an Allan deviation of 30 kHz over 1 second and <80 kHz over 1 hour. The scheme is very robust and affordable, and it would be ideal for carrying out a range of quantum information experiments.     

Resonance transition 795-nm rubidium laser using He buffer gas

We report a demonstration of a 795-nm rubidium optical resonance transition laser using a buffer gas consisting of pure ³He. This follows our recent demonstration of a hydrocarbon-free 795-nm rubidium resonance laser which used naturally-occurring He as the buffer gas. Using He gas that is isotopically enriched with ³He yields enhanced mixing of the Rb fine-structure levels. This enables efficient lasing at reduced He buffer gas pressure, improved thermal management in high average power Rb lasers and enhanced power scaling potential of such systems.     

Growth and properties of KLu(WO4)2, and novel ytterbium and thulium lasers based on this monoclinic crystalline host

High‐quality crystals of monoclinic KLu(WO₄)₂, shortly KLuW, were grown with sizes sufficient for its characterization and substantial progress was achieved in the field of spectroscopy and laser operation with Yb³⁺‐ and Tm³⁺‐doping. We review the growth methodology for bulk KLuW and epitaxial layers, its structural, thermo‐mechanical, and optical properties, the Yb³⁺ and Tm³⁺ spectroscopy, and present laser results obtained in several operational regimes both with Ti:sapphire and direct diode laser pumping using InGaAs and AlGaAs diodes near 980 and 800 nm, respectively. The slope efficiencies with respect to the absorbed pump power achieved with continuous‐wave (CW) bulk and epitaxial Yb:KLuW lasers under Ti:sapphire laser pumping were ≈ 57 and ≈ 66%, respectively. Output powers as high as 3.28 W were obtained with diode pumping in a simple two‐mirror cavity where the slope efficiency with respect to the incident pump power reached ≈ 78%. Passively Q‐switched laser operation of bulk Yb:KLuW was realized with a Cr:YAG saturable absorber resulting in oscillation at ≈ 1031 nm with a repetition rate of 28 kHz and simultaneous Raman conversion to ≈ 1138 nm with maximum energies of 32.4 and 14.4 μJ, respectively. The corresponding pulse durations were 1.41 and 0.71 ns. Passive mode‐locking by a semiconductor saturable absorber mirror (SESAM) produced bandwidth‐limited pulses with duration of 81 fs (1046 nm, 95 MHz) and 114 fs (1030 nm, 101 MHz) for bulk and epitaxial Yb:KLuW lasers, respectively. Slope efficiency as high as 69% with respect to the absorbed power and an output power of 4 W at 1950 nm were achieved with a diode‐pumped Tm:KLuW laser. The slope efficiency reached with an epitaxial Tm:KLuW laser under Ti:sapphire laser pumping was 64 %. The tunability achieved with bulk and epitaxial Tm:KLuW lasers extended from 1800 to 1987 nm and from 1894 to 2039 nm, respectively.     

High-resolution laser spectroscopy of ultracold ytterbium atoms using spin-forbidden electric quadrupole transition

We have successfully observed high-resolution spectra of spin-forbidden electric quadrupole transition (¹ S ₀→³ D ₂) in ytterbium (¹⁷⁴Yb) atoms. The differential light shifts between the ¹ S ₀ and the ³ D ₂ states in a far-off resonant trap at 532 nm are also measured. For the spectroscopy, we developed simple, narrow-linewidth, and long-term frequency stabilized violet diode laser systems. Long-term drifts of the excitation laser (404 nm) is suppressed by locking the laser to a length stabilized optical cavity. The optical path length of the cavity is stabilized to another diode laser whose frequency is locked to a strong ¹ S ₀→¹ P ₁ transition (399 nm) of Yb. Both lasers are standard extended-cavity diode lasers (ECDLs) in the Littrow configuration. Since the linewidth of a violet ECDL (～10 MHz) is broader than a typical value of a red or near infra-red ECDL (<1 MHz), we employ optical feedback from a narrow-band Fabry–Perot cavity to reduce the linewidth. The linewidth is expected to be <20 kHz for 1 ms averaging time, and the long-term frequency stability is estimated to be ～200 kHz/h.