Generation of ultrafast mid-infrared laser by DFG between two actively synchronized picosecond lasers in a MgO:PPLN crystal

We report the difference-frequency generation (DFG) of ultrafast mid-infrared laser radiation around 3???m between two picosecond laser pulses with the center wavelengths of 800?nm and 1064?nm in a MgO:PPLN crystal at room temperature. The two laser pulses were generated from the actively synchronized picoseconds Ti:sapphire and Nd:YVO₄ oscillators. We measured the DFG wavelengths tunable from 3.19?C3.29???m and the output power is potential to be several mW. This experiment proves a possible roadmap for ultrafast mid- and far-infrared laser radiation generation and even for the THz radiation.     

Energy Scaling of Terahertz Pulses Produced through Difference Frequency Generation

We study the energy scaling of terahertz(THz) emission through difference frequency generation of near-infrared pulses, and demonstrate that Gigawatt few-cycle THz transients at the central frequency of 30 THz are produced from GaSe crystal pumped by two pulses at 1.65 and 1.95 micrometers, with the high quantum yield of 28%.Our analysis indicates that the high yield of DFG originates from the largely reduced group velocity mismatch as the long-wavelength pumping pulses are employed.     

Optimization of the idler wavelength tunable cascaded optical parametric oscillator based on chirp-assisted aperiodically poled lithium niobate crystal

We present the numerical results for the optimization of the pump-to-idler conversion efficiencies of nanosecond idler wavelength tunable cascaded optical parametric oscillators(OPO) in different wavelength tuning ranges, where the primary signals from the OPO process are recycled to enhance the pump-to-idler conversion efficiencies via the simultaneous difference frequency generation(DFG) process by monolithic aperiodically poled, magnesium oxide doped lithium niobate(APMg LN) crystals. The APMg LN crystals are designed with different chirp parameters for the DFG process to broaden their thermal acceptance bandwidths to different extents. The idler wavelength tuning of the cascaded OPO is realized by changing the temperature of the designed APMg LN crystal and the cascaded oscillation is achieved in a single pump pass singly resonant linear cavity. The pump-to-idler conversion efficiencies with respect to the pump pulse duration and ratio of OPO coefficient to DFG coefficient are calculated by numerically solving the coupled wave equations. The optimal working conditions of the tunable cascaded OPOs pumped by pulses with energies of 350 μJ and 700 μJ are compared to obtain the general rules of optimization. It is concluded that the optimization becomes the interplay between the ratio of OPO coefficient to DFG coefficient and the pump pulse duration when the idler wavelength tuning range and the pump pulse energy are fixed. Besides, higher pump pulse energy is beneficial for reaching higher optimal pump-to-idler conversion efficiency as long as the APMg LN crystal is optimized according to this pump condition. To the best of our knowledge,this is the first numerical analysis of idler wavelength tunable cascaded OPOs based on chirp-assisted APMg LN crystals.     

基于飞秒锁模光纤激光脉冲基频光的差频产生红外光梳

报道了一种基于飞秒锁模光纤激光脉冲基频光的光纤型差频产生(DFG)红外光梳及其研制技术.基于自主研制的重频锁定200 MHz飞秒锁模掺铒光纤激光器,经啁啾脉冲光纤放大与超连续谱产生技术,优化近零色散OFS光纤(型号:OFS-980-20)长度,结合可调延时线,获得了精准同步的基频双色脉冲;以GaSe为非线性晶体,利用光整流技术,产生了可在6—10μm范围内宽带调谐的DFG红外光梳,光梳最大光谱宽度可达1.3μm.这种光纤型远红外光梳可望在分子光谱精密测量等领域发挥重要作用.     

Difference-Frequency Generation Among Ultrashort Optical Pulses in Quasi-Phase-Matching Waveguides

A theoretical model of ultrashort pulse difference-frequency generation (DFG) is presented and developed with quasi-phase matching (QPM) gratings in the undepleted-pump, unamplified-signal approximation. An analytic solution to a case of ultrashort pulse pumped DFG process, including group-velocity mismatching effects and input pulses with frequency chirp and time delay, is obtained. The influences of group-velocity mismatching effects and input signal pulse parameters on the conversion efficiency and output converted pulse characteristics are analyzed and discussed. The results indicate that the conversion efficiency is increased due to the enhancement of pump and signal interaction. The output pulse is inevitable compressed under pulsed pumping and can be compensated by introducing the initial frequency chirp and time delay.     

Difference-frequency generation by mixing dual-wavelength pulses emitting from an electronically tuned Ti:sapphire laser

Broadly tunable difference-frequency generation (DFG) in AgGaS₂ was achieved by mixing dual-wavelength oscillating pulses from an electronically tuned Ti:sapphire laser with a two-frequency-driven acousto-optic device. Continuous tuning from 6.5 to 8.5 μm was achieved by simultaneous dual-wavelength-tuned DFG without crystal rotation. In the dual-pulse oscillation, the shorter and longer wavelength pulses were tuned from 700 to 775 nm and from 763 to 880 nm, respectively, while keeping the phase-matching relationship for DFG. When crystal rotation was adopted, however, the tunable output range was extended from 5.3 to 12 μm by tuning the longer wavelength pump pulse, while the shorter wavelength pulse was fixed. Received: 18 November 1998 / Revised version: 5 February 1999 / Published online: 26 May 1999     

Ultrabroadband self-phase-stabilized pulses by difference-frequency generation

Ultrabroadband near-IR (800-1700-nm) pulses are obtained by type II difference-frequency generation (DFG) between two synchronized noncollinear optical parametric amplifiers. Self-stabilization of the carrier-envelope offset phase, as expected from the DFG process, is demonstrated experimentally.     

Nonlinear optical terahertz wave sources

We developed a Cherenkov phase-matching method for monochromatic THz-wave generation using the DFG, process with a lithium niobate crystal, which resulted in both high conversion efficiency and wide tunability. Although THz-wave generation by Cherenkov phase matching has been demonstrated using femtosecond pumping pulses, producing very high peak power, these THz-wave sources are not monochromatic. Our method generates monochromatic and tunable THz, waves using a nanosecond pulsed laser source. We also show that Cherenkov radiation with waveguide structure is an effective strategy for achieving extremely wide tunable THz-wave source. We fabricated MgO-doped lithium niobate slab waveguide and demonstrated difference frequency generation of THz-wave generation with Cherenkov phase matching. Extremely frequency-widened THz-wave generation, from 0.1 to 7 THz was observed.     

Carrier-envelope phase offset for pulses from a tunable optical parametric amplifier

The carrier-envelope phase (CEP) characteristics of the tunable infrared laser pulses from a noncollinear optical parametric amplifier (OPA) with passively stabilized CEP are investigated experimentally. We compare the CEP fluctuation of different wavelength outputs from the OPA which is seeded by the idler pulse of a difference frequency generation (DFG) process. It is found that when the OPA output is tuned to a longer wavelength, the CEP fluctuation becomes less sensitive to the jitter of laser intensity and the phase mismatch, and therefore more stable CEP for the longer wavelength output pulses is realized.     

Single attosecond pulses from high harmonics driven by self-compressed filaments

We show that isolated subfemtosecond, extreme ultraviolet (XUV) pulses can be generated via harmonic generation in argon by few-cycle infrared pulses formed through filamentation-induced self-compression in neon. Our calculations show that the time structure of the XUV pulses depends sensitively on both the amplitude and the phase modulation that are induced in the driving pulse during the self-compression process.     

Inhibiting three-body recombination in atomic Bose-Einstein condensates

We discuss the possibility of inhibiting three-body recombination in atomic Bose-Einstein condensates via the application of resonant 2pi laser pulses. These pulses result in the periodic change in the phase of the molecular state by pi, which leads to destructive interference between the decay amplitudes following successive pulses. We show that the decay rate can be reduced by several orders of magnitude under realistic conditions.     

Spectral amplitude and phase measurement of ultrafast pulses using all-optical differential tomography

We demonstrate a simple, all-optical, fiber-based method for characterizing the spectral amplitude and phase of ultrafast pulses using a differential tomographic measurement realized via four-wave mixing. The technique is applied to subpicosecond pulses in the C-band of the telecommunication spectrum. Characterization of amplified pulses and propagation through dispersive media is demonstrated and compared with autocorrelation measurements and calculated predictions. We show how our approach can be extended to larger bandwidths in similar systems, extending tomographic reconstruction of coherent fields to nearly an octave of bandwidth while maintaining a robust, waveguide-based geometry.     

Running pulses of complex shape in a reaction-diffusion model

In a one-dimensional reaction-diffusion model of an active medium, stable steady-state wave pulses of a new type are described. They are called multihumped because their waveforms contain several maxima of similar size. Presumably, the multihumped pulses arise via a bifurcation at which an unstable trigger wave disappears. The parameter governing this bifurcation is the diffusion coefficient for the model inhibitor. The model is analyzed by varying this parameter to determine the conditions for the emergence of multihumped pulses. The results of this analysis show how their waveform and dynamics of excitation depend on the inhibitor diffusion coefficient.     

Tunable mid-infrared,high-energy femtosecond laser source for glyco-protein structure analysis

We have developed a 6–12 μm mid-infrared (MIR) femtosecond laser source for glyco-protein structure analysis. The MIR femtosecond laser pulses are generated by a differential frequency generation (DFG) configuration with a combination of Ti:sapphire based regeneratively amplified femtosecond laser pulses (780 nm, 160 fs, 1 mJ) and a β-BaB₂O₄ (BBO) based optical parametric amplifier (OPA). The MIR pulse energy exceeds 4.5 μJ, where a glyco-protein molecule has resonant absorption lines due to the vibrational–rotational transitions. The pulse width is estimated to be less than 1 ps according to the cross correlation measurement between the two OPA output pulses. Using the MIR femtosecond laser pulses, we demonstrated photo-dissociation of the sialyl Lewis X (sLeX) proton added ion, which is the first time to the best of our knowledge. PACS 42.65.Re; 42.62.-b; 42.60.-b; 42.65.-k; 87.50     

Double quasi phase matching for both optical parametric oscillator and difference frequency generation

We present simultaneous phase matching of optical parametric oscillator (OPO) and difference frequency generation (DFG), using a noncollinear interaction in periodically poled crystal with single grating. Selecting proper grating period Λ and titled angle ξ between the grating vector G and the optical axis of crystal, the noncollinear scheme provides double phase matching solutions over continuous regions of the midwave infrared spectrum. At certain wavelength regions, for DFG process the group velocities between interaction pulses are matching and the phase matching bandwidth reaches maximum. Selecting the different grating period, the broadband midwave tuning and better gain spectrum can be obtained at different wavelength range. For the certain period grating the conversion efficiency is higher. Hence, using the double phase matching configuration, the broadband tunable midwave infrared wave can be produced in single grating. But the configurations have a relatively narrow angular bandwidth.     

Reduction of light signal pulse distortion in cascaded sum-frequency-generation and difference-frequency-generation wavelength conversion

Cascaded sum-frequency-generation (SFG) and difference-frequency-generation (DFG) can implement a wavelength conversion between arbitrary combinations of input and output signal wavelengths. By using a tunable wavelength pump light, the output wavelength can be tuned to a desired wavelength. As in many wavelength conversion devices using the nonlinear optical effect, the group velocity difference between light pulses with different wavelength causes a walk-off effect deforming the output pulse shape. Thus the device length should be kept short to avoid the walk-off effect resulting in limited conversion efficiency. In this report, we propose a method for a quasi-phase matched (QPM) device to maintain the pulse shape of the SFG light pulse along the propagation distance. The output DFG light pulse deformation is suppressed and the conversion efficiency can be increased by extending the device length.     

Experimental observation of tunable wavelength down- and up-conversions of ultra-short pulses in a periodically poled LiNbO3 waveguide

All-optical tunable wavelength conversion of ps-pulses is proposed and experimentally demonstrated by use of cascaded sum- and difference frequency generation (cSFG/DFG) in a periodically poled LiNbO₃ (PPLN) waveguide. The amplified spontaneous emission (ASE) noise is effectively suppressed by employing two tunable filters. As a result, tunable wavelength down- and up-conversions are simultaneously observed. The temporal evolutions of the signal, pump, control and idler waves propagating along the PPLN waveguide are simulated. From the temporal waveforms and optical spectra in the simulations, it is interesting to find that continuous wave (CW) pump and control are evolved into optical pulses during the cSFG/DFG nonlinear interactions. Moreover, some new sidebands in the output pump spectrum are observed both in the simulations and experiments.     

Normal group-velocity dispersion Kerr frequency comb

We show via numerical simulation that Kerr frequency combs can be generated in a nonlinear resonator characterized with normal group-velocity dispersion. We find the spectral shape of the comb and temporal envelope of the corresponding optical pulses formed in the resonator.     

Spatiotemporal toroidal waves from the transverse second-harmonic generation

We study the second-harmonic generation via transversely matched interaction of two counterpropagating ultrashort pulses in chi(2) photonic structures. We show that the emitted second-harmonic wave attains the form of spatially expanding toroid with the initial thickness given by the cross correlation of the pulses. We demonstrate the formation of such toroidal waves in crystals with random ferroelectric domains as well as in annularly poled nonlinear photonic structures.     

Metal nanoplasmas as bright sources of hard X-ray pulses

We report significant enhancements in light coupling to intense-laser-created solid plasmas via surface plasmon and "lightning rod" effects. We demonstrate this in metal nanoparticle-coated solid targets irradiated with 100 fs, 806 nm laser pulses, focused to intensities approximately 10(14)-10(15) W cm(-2). Our experiments show a 13-fold enhancement in hard x-ray yield (10-200 keV) emitted by copper nanoparticle plasmas formed at the focal volume. A simple model explains the observed enhancement quantitatively and provides pointers to the design of structured surfaces for maximizing such emissions.