Nuclear magnetic moment of the 9.7 h 12− isomer 196mAu

The magnetic hyperfine splitting v_M=|gμ_NB_HF/h| of ^196mAu (j^π=12^?; configuration ¦(π$\text{11}\text{2}$($\text{v}\text{13}\text{2}{}^{\mathrm{+}}\text{)〉}{}_{12}{}^{\mathrm{?}}$; $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 9.7}\text{h}\text{)}$ as dilute impurity in Ni has been determined with nuclear magnetic resonance on oriented nuclei as 96.0(2) MHz. With the known hyperfine field B_HF = ?264.4(3.9) kG corrected for hyperfine anomalies the g-factor and magnetic moment of ^196mAu are deduced to be |g| = 0.476(7) and |μ| = 5.72(8) μ_N. Taking into account the known magnetic properties of $\text{π}\text{1}\text{2}{}^{\mathrm{?}}$ and $\text{v}\text{13}\text{2}{}^{\mathrm{+}}$ isomeric states in the neighbouring odd Pt, Au and Hg nuclei the structure of the 12^? state is discussed.     

The g-factor of the72+[404] ground state of 177Ta

With the technique of nuclear magnetic resonance on oriented nuclei the hyperfine splitting $\text{ν}{}_{\mathrm{<mtext>M</mtext>}}\text{= ¦gμ}{}_{\mathrm{<mtext>N</mtext>}}\text{B}{}_{\mathrm{<mtext>HF</mtext>}}\text{/h¦}\text{of}{}^{177}\text{Ta}\text{(j}{}^{\mathrm{\pi }}\text{7}\text{2}{}^{\mathrm{+}}\text{; T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 56.6h)}$ in Fe has been measured With the known hyperfine field $\text{B}{}_{\mathrm{<mtext>HF</mtext>}}\text{(}\text{Ta}\text{Fe}\text{) = ?648 (13)}\text{kG the}\text{g-}\text{factor of the}\text{7}\text{2}{}^{\mathrm{+}}\text{[404]}$ ground state of ¹⁷⁷Ta is deduced to be $\text{¦g¦ = 0.643 (13)}$.     

Nuclear magnetic moment of the 3.9 s112− isomer 193mAu

The magnetic hyperfine splitting ν_M = |gμ_NB_HF/h| of ${}^{\mathrm{<mtext>193</mtext><mtext>m</mtext>}}\text{Au}\text{(j}{}^{\mathrm{\pi }}\text{=}\text{11}\text{2}{}^{\mathrm{?}}\text{, E = 290}\text{keV}$; $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 3.9}\text{s}\text{)}$ as a dilute impurity in Ni has been measured with nuclear magnetic resonance on oriented nuclei as 226.4(2) MHz. With the known hyperfine field B_HF = ?264.4(3.9) kG corrected for hyperfine anomalies the g-factor and magnetic moment of ^193mAu are deduced to be |g| = 1.123(17) and |μ| = 6.18(9) μ_N.     

Measurement of the magnetic moment of the 7+ isomer in 198Tl

Using the atomic beam magnetic resonance method the hyperfine structure separation of $\text{1.9}\text{h}{}^{\mathrm{198m}}\text{Tl}\text{(I}{}^{\mathrm{\pi }}\text{= 7}{}^{\mathrm{+}}\text{)}$ has been measured in the ${}^2\text{P}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}$ atomic ground state. From the hyperfine structure splitting the nuclear magnetic dipole moment has been deduced. The results are: Δν = 4500 (68) MHz, μ_I = 0.641(10)μ_N. This is an improvement of approximately one order of magnitude compared to a previous measurement. The quoted value of the magnetic dipole moment includes corrections for the hyperfine structure anomaly and for diamagnetic shielding.     

Nuclear moments of the low abundant natural isotope 176Lu and hyperfine anomalies in the lutetium isotopes

The atomic beam magnetic resonance method combined with laser-induced state- and isotopeselective detection of metastable atoms has been used to investigate the hyperfine structure of the ²D ground multiplet in ¹⁷⁵Lu and ¹⁷⁶Lu. The analysis of the data yields not only accurate values for the hyperfine interaction constants, the nuclear magnetic dipole moment of ¹⁷⁵Lu, and the electronic g_J, factors, but also the first directly measured value of the nuclear magnetic dipole moment of the low abundant isotope ${}^{176}\text{Lu}\text{: μ}{}_{\mathrm{I}}\text{(}{}^{176}\text{Lu) = 3.1692 (45)μ}{}_{\mathrm{<mtext>N</mtext>}}$ (corrected for diamagnetic shielding). The spectroscopic quadrupole moment of ¹⁷⁶Lu was calculated from the ratio of the B-factors and the quadrupole moment of ${}^{175}\text{Lu}\text{: Q}{}_{\mathrm{<mtext>s</mtext>}}\text{(}{}^{176}\text{Lu}\text{) = 4.92 (3)}\text{b}$. Moreover, the magnetic hyperfine anomalies for the isotopic chain ^{175,176,176m,177}Lu were determined. A quadrupole hyperfine anomaly between ¹⁷⁵Lu and ¹⁷⁶Lu was not found when comparing the ratio of the B-factors in the states ${}^2\text{D}{}_{\mathrm{<mtext>3</mtext><mtext>2</mtext>}}\text{and}{}^2\text{D}{}_{\mathrm{<mtext>5</mtext><mtext>2</mtext>}}$. From a comparison of the quadrupole moment of ¹⁷⁵Lu obtained from the hyperfine structure data and the quadrupole moment measured in muonic lutetium atoms semi-empirical Sternheimer shielding factors could be estimated.     

g-factors of 2.7 h 93Tc, 4.9 h 94Tc and 20 h 95Tc

The hyperfine splitting frequencies gμ_NB_H.F./h of 2.7 h ⁹³Tc $\text{(J}{}^{\mathrm{\pi }}\text{=}\text{9}\text{2}{}^{\mathrm{+}}\text{)}$, 4.9 h ⁹⁴Tc (J^π = 7⁺) and 20 h ⁹⁵Tc $\text{(J}{}^{\mathrm{\pi }}\text{=}\text{9}\text{2}{}^{\mathrm{+}}\text{)}$ as dilute impurities in Fe have been measured with NMR on oriented nuclei as 336.36(5) MHz, 175.11(1) MHz and 315.97(2) MHz, respectively. From the resonance shifts with an external magnetic field B₀ the hyperfine field of Tc$\text{Fe}$ has been determined as -317(5) kG. Taking this into account the nuclear g-factors are deduced as $\text{g(}{}^{93}\text{Tc}\text{) = 1.392(22), g(}{}^{94}\text{Tc}\text{) = 0.725(11)}\text{and}\text{g(}{}^{95}\text{Tc}\text{) = 1.308(21)}$.     

Susceptibilities of the S = 12 XY model on the square lattice at T = 0

For the $\text{S =}\text{1}\text{2}\text{XY}$ model at T = 0 four susceptibilities have been calculated exactly on a sequence of finite square lattices and extrapolated to the infinite square lattice. For the ferromagnet χ_zz = 0 while χ_xx ～ N^2.9; for the antiferromagnet $\text{J}{}_{\mathrm{\chi xx}}\text{N(gμ}{}_{\mathrm{<mtext>B</mtext>}}\text{)}{}^2\text{= 0.025 ± 0.002}$ and $\text{J}{}_{\mathrm{\chi xx}}\text{N(gμ}{}_{\mathrm{<mtext>B</mtext>}}\text{)}{}^2\text{= 0.13 ± 0.03}$.     

Determination of the spectroscopic quadrupole moments of 131Cs, 132Cs and 136Cs

Nuclear spectroscopic quadrupole moments of the radioactive isotopes ¹³¹Cs, ¹³²Cs, and ¹³⁶Cs have been determined from the hyperfine structure of the $\text{6}{}^2\text{P}{}_{\mathrm{<mtext>3</mtext><mtext>2</mtext>}}$ state by the level crossing method. The results including a Sternheimer correction are: $\text{Q}{}_{\mathrm{<mtext>s</mtext>}}\text{(}{}^{131}\text{Cs}\text{) = ?0.625(6)}\text{b}$, $\text{Q}{}_{\mathrm{<mtext>s</mtext>}}\text{(}{}^{132}\text{Cs}\text{) = +0.508(7)}\text{b}$, $\text{Q}{}_{\mathrm{<mtext>s</mtext>}}\text{(}{}^{136}\text{Cs}\text{) = +0.225(10)}\text{b}$. The quadrupole moments of all the Cs isotopes from A = 131 to A = 137 are recalculated. It is shown, that nuclear quadrupole moments of a specific isotope obtained from different atomic P-states only agree within the limits of error after application of the Sternheimer correction. The increase of Q_s with decreasing neutron number conforms with other observations and theoretical calculations stating that for elements around Z = 55 nuclear deformation develops below N = 82. The staggering of the sign of Q_s may be interpreted as consequence of an oblate-prolate degeneracy of the nuclear energy surface. Some magnetic moments have been slightly improved: $\text{μ}{}_{\mathrm{<mtext>I</mtext>}}\text{(}{}^{132}\text{Cs}\text{) = 2.219(7) μ}{}_{\mathrm{<mtext>N</mtext>}}$, $\text{μ}{}_{\mathrm{<mtext>I</mtext>}}\text{(}{}^{136}\text{Cs}\text{) = 3.705(15)μ}{}_{\mathrm{<mtext>N</mtext>}}$ (corrected for diamagnetism).     

Magnetic moments at backbending and spectroscopy of 134Ce

Employing the static hyperfine fields at cerium nuclei in magnetized Fe and Gd hosts, the g-factor of the ¹³⁴Ce(10⁺) state at backbending (E_{x = 3719.3 keV}) has been determined as g = ? 0.30 (25). The coexistence of this neutron-dominated state with the ($\text{v}\text{h}{}_{\mathrm{<mtext>11</mtext><mtext>2</mtext>}}\text{)}{}^{\mathrm{n}}\text{10}{}^{\mathrm{+}}$ isomer (E_x = 3208.5 keV, g = ?0.19(1)) is unexpected. A comprehensive spectroscopic study following the ¹²²Sn(¹⁶O, 4n) reaction, including γ-angular distributions, prompt and delayed γ coincidence and recoil-distance measurements has yielded new information on quasi-collective bands of both parities. The properties of the low-lying positive-parity states are well described by the interacting boson model.     

The emission spectra of H35Cl+, H37Cl+, D35Cl+, and D37Cl+ in the region 2700–4100 Å

The $\text{A}{}^2\text{Σ}{}^{\mathrm{+}}\text{-X}{}^2\text{Π}$ emission spectrum of HCl⁺ has been measured and analyzed for four isotopic combinations. These analyses extend previous work and provide rotational constants for the v = 0–2 levels of the ground state and for the v = 0–9 levels of the excited state. RKR potentials have been determined for both states, although the upper state could not be fitted precisely to such a model. Calculated relative intensities based on these potentials demonstrated that the electronic transition moment must change rapidly with lower state vibrational quantum number. Although considerable caution should be exercised in applying the concept of equilibrium constants to the $\text{A}{}^2\text{Σ}{}^{\mathrm{+}}$ state, the following are the best estimates of these constants (in cm^?1) for the $\text{X}{}^2\text{Π}$ state of H³⁵Cl⁺: B_e = 9.9406, ω_e = 2673.7, A_e = ? 643.7, and $\text{r}{}_{\mathrm{e}}\text{= 1.315}\text{A}\text{?}$. For the $\text{A}{}^2\text{Σ}{}^{\mathrm{+}}$ state of H³⁵Cl: T_e = 28 628.08, B_e ～ 7.505, ω_e ～ 1606.5, and $\text{r}{}_{\mathrm{e}}\text{= 1.514}\text{A}\text{?}$.     

The g-factor difference for the 61+ and 88+ states in 210Po

The difference in g-factors for the 6₁⁺ and 8₁⁺$\text{(πh}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}{}^2\text{)}$ states in ²¹⁰Po has been measured as $\text{(g}{}_6\text{? g}{}_8\text{)}\text{g}{}_8\text{= 2.0 ± 0.7\%}$. This result represents a small violation of additivity. A value of g₈ = 0.909 ± 0.011, independent of g₆, was also obtained.     

The spectrum of HeNe+

Discharges through mixtures of helium and neon show two band groups near 4250 and 4100 Å as first observed by Druyvesteyn. These bands, assigned to the HeNe⁺ ion by Tanaka, Yoshino, and Freeman, have been studied under high resolution and have been fairly completely analyzed. The upper state of the transition is a very weakly bound state resulting from $\text{He}{}^{\mathrm{+}}\text{(}{}^2\text{S) +}\text{Ne}\text{(}{}^1\text{S}{}_0\text{)}$. There are two lower states resulting from the two components of $\text{Ne}{}^{\mathrm{+}}\text{(}{}^2\text{P) +}\text{He}\text{(}{}^1\text{S}{}_0\text{)}$. The upper of these two (${}^2\text{Π}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}$) is also very weakly bound while the lower of the two, the ²Σ⁺ ground state, has a dissociation energy of 0.69 eV and an r_e value of 1.30 Å. All bands in both band groups show four branches designated R_ff, Q_ef, Q_fe, and P_ee. From their analysis the rotational constants in the various vibrational levels of the three electronic states have been determined. While no spin splitting in the B²Σ⁺ state has been found the ground state X²Σ shows a very large spin splitting and the $\text{A}{}_2{}^2\text{Π}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}$ state a very large $\text{Ω-type}$ doubling. The vibrational numberings in all these states were established by the study of the spectrum of ³HeNe⁺. At the same time the hyperfine structure observed in all lines of ³HeNe⁺ confirmed the nature of the upper state B²Σ⁺ as resulting from He⁺ + Ne, i.e., by charge exchange from the ground state. The ${}^2\text{Π}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}$ component of the ²Π state has not been observed, presumably because of low intensity.     

Polarization spectroscopy of the E0g+-B0u+ band system of Br2

The E-B (0_g⁺-0_u⁺) band system of Br₂ has been investigated at Doppler-limited resolution using polarization labeling spectroscopy. Merged E state data for the three naturally occurring isotopes in the range v_E = 0–16, expressed in terms of the constants for ⁷⁹Br₂, are (in cm^?1) Y_0,0 = 49 777.962(54), Y_1,0 = 150.834(22), Y_2,0 = ?0.4182(28), Y_3,0 = 6.6(11) × 10^?4, Y_0,1 = 4.1876(28) × 10^?2, Y_1,1 = ?1.607(16) × 10^?4, and Y_0,2 = 1.39(39) × 10^?8. The bond distance is $\text{r}{}_{\mathrm{<mtext>e</mtext>}}\text{= 3.194}\text{A}\text{?}$, and the diabatic dissociation energy to $\text{Br}{}^{\mathrm{+}}\text{(}{}^3\text{P}{}_2\text{) +}\text{Br}{}^{\mathrm{?}}\text{(}{}^1\text{S}{}_0\text{)}\text{is 34 700 cm}{}^{\mathrm{?1}}$.     

Structural connections between 148Sm and 149Sm nuclei

The ^{146, 148}Nd(α, χn) and ^{148, 150}Nd(³He, χn) reactions at E_α = 20–43 MeV and E_3He = 19–27 MeV, are used to study excited states in the ¹⁴⁹Sm₈₆ and ¹⁴⁹Sm₈₇ nucleides and consequently the low-spin odd-parity excitation. The mixing ratios and multipolarities of the most prominent transitions are deduced from the combined evidence of angular distribution and electron conversion data. The spin-parity assignments for most of the levels observed are established. In ¹⁴⁸Sm the ground state band extending to I^π = 10⁺ is predominantly populated. A negative-parity odd-spin band extending from I^π = 3^?through 11^? is also observed. The bands in ¹⁴⁸Sm are interpreted within the framework of the interacting boson approximation model. In ¹⁴⁹Sm positive-parity levels with spin up to $\text{25}\text{2}$ and negative-parity levels with spins up to $\text{21}\text{2}$ are observed. The predominant γ-decay proceeds via transitions associated with $\text{i}{}_{\mathrm{<mtext>13</mtext><mtext>2</mtext>}}$, $\text{h}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}$, $\text{f}{}_{\mathrm{<mtext>7</mtext><mtext>2</mtext>}}$ and $\text{h}{}_{\mathrm{<mtext>11</mtext><mtext>2</mtext>}}$ intrinsic configurations. The branching ratios B(E1)/B(E2) are calculated and compared in both ¹⁴⁸Sm and ¹⁴⁹Sm nucleides. The B(E1)/B(E2) dependence on the value of Z for some N = 86 (as well as 88 and 84) isotones showing a minimum of Z = 64 was noted. A 4 ns high-spin isomer mainly decaying into the positive-parity band based on the $\text{i}{}_{\mathrm{<mtext>13</mtext><mtext>2</mtext>}}$ state in ¹⁴⁹Sm is found. Experimental evidence is presented to interprete the $\text{1}\text{2}{}^{\mathrm{+}}$, $\text{15}\text{2}{}^{\mathrm{+}}$, … and $\text{9}\text{2}{}^{\mathrm{?}}$, $\text{13}\text{2}{}^{\mathrm{?}}$, …, ΔI = 2, sequences in ¹⁴⁹Sm as arising from the coupling of an $\text{h}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}$ neutron to the octupole and quadrupole modes of the ¹⁴⁸Sm core nucleus. The absolute reaction cross sections for the ^{146, 148, 150}Nd(³He, χn) reactions have been determined for different bombarding energies. The mixing of the $\text{f}{}_{\mathrm{<mtext>7</mtext><mtext>2</mtext>}}$ and $\text{h}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}$ shells is discussed in the framework of an axial-particle-rotor model calculation.     

Tabulation of hyperfine splittings in rotational F1 and F2 levels of the ground vibrational state of 12CH4 for J ≤ 20

To a good approximation, hyperfine splittings for F₁ and F₂ rotational levels of the ground vibrational state of ¹²CH₄ depend linearly on three hyperfine interaction parameters. Coefficients in these linear expressions have been computed in a relatively simple manner and tabulated for levels with 1 ≤ J ≤ 20. The hyperfine pattern for the $\text{J = 7 F}{}_2{}^{\mathrm{(2)}}$ level computed from these expressions using values for the three hyperfine interaction parameters reported recently by Yi, Ozier and Ramsey (1) agrees well with the pattern obtained from new HeNe laser measurements of Hall and Bordé (2) on the $\text{P(7) F}{}_2{}^{\mathrm{(2)}}$ line of the ν₃ band of methane.     

Energy levels of low lying triplet states of N2 from infrared emission studies

A theoretical model used to describe the $\text{B′}{}^3\text{Σ}{}_{\mathrm{u}}{}^{\mathrm{?}}$ and B³Π_g states of N₂ is presented. Using recently acquired high resolution spectra of the $\text{B′}{}^3\text{Σ}{}_{\mathrm{u}}{}^{\mathrm{?}}\text{→ B}{}^3\text{Π}{}_{\mathrm{g}}$ (0-0) band, rotational energy levels of the v = 0 vibrational levels of these two states are generated with this model. These levels are in excellent agreement with those obtained using a combination differences technique. The precision of the model generated levels is 0.01 cm^?1. The previously unpublished rotational levels of Dieke and Heath for the $\text{A}{}^3\text{Σ}{}_{\mathrm{u}}{}^{\mathrm{+}}$, B³Π_g and C³Π_u states are referenced to the $\text{N}{}_2\text{X}{}^1\text{Σ}{}_{\mathrm{g}}{}^{\mathrm{+}}$ (v = 0, J = 0) ground level and tabulated here. Estimates of the precision of their work are made.     

The decay process 11ΛB → π− + 11C

The branching ratios are calculated for ¹¹_ΛB decay to the ¹¹C ground and excited states below 8 MeV for two possible spin values of ¹¹_ΛB. It is found that the decay rate to the ¹¹C^★ state at E^★ = 6.48 MeV is comparable in magnitude to that leading to the ¹¹C ground state if $\text{J(}{}^{11}{}_{\mathrm{\Lambda }}\text{B}\text{) =}\text{5}\text{2}$ is assumed. This result, unlike the branching ratios calculated for the $\text{J(}{}^{11}{}_{\mathrm{\Lambda }}\text{B}\text{) =}\text{7}\text{2}$ case, is in accord with experiment and lends support to the assumption that $\text{J =}\text{5}\text{2}$ holds for ¹¹_ΛB. The necessity of the reinterpretation of some of the so-called ¹³_ΛC events in terms of ${}^{11}{}_{\mathrm{\Lambda }}\text{B}\text{→ π}{}^{\mathrm{?}}\text{+}{}^{11}\text{C}{}^1$ is indicated.     

Oblate ground-state shapes of 11 h 189Pt and 2.8 d 191Pt

With nuclear orientation on $\text{11}\text{h}\text{3}\text{2}{}^{\mathrm{?189}}\text{Pt}\text{, 2.8}\text{d}\text{3}\text{2}{}^{\mathrm{?191}}\text{Pt}$ and $\text{4.0}\text{d}\text{13}\text{2}{}^{\mathrm{<mtext>+\; 195\; </mtext><mtext>m</mtext>}}\text{Pt}$ in Os and NMR on oriented ¹⁸⁹Pt and ¹⁹¹Pt in Fe electric and magnetic hyperfine splitting frequencies were measured. The nuclear moments are deduced to be: ¹⁸⁹Pt: |μ| = 0.434(9) μ_N, Q = ?0.65(26) b; ¹⁹¹Pt: |μ| = 0.500(10) μ_N, Q = ?0.64(26) b; ^195mPt: Q = +1.42(60)b. The negative spectroscopic ground-state quadrupole moments of ¹⁸⁹Pt and ¹⁹¹Pt must be due to oblate ground-state deformations, thus indicating that the prolate-oblate phase transition in Pt is located at A < 189.     

Average polarization of 12B in 12C(μ, ν)12B(g.s.) reaction: Helicity of the π-decay muon and nature of the weak coupling

The helicity, h^?, of μ^? in π-decay has been determined as positive (h^??+0.90) from the average polarization, P_av≡〈J_B·s_μ〉, of ¹²B produced in the $\text{μ}{}^{\mathrm{?}}\text{+}{}^{12}\text{C}\text{→ν}{}_{\mathrm{\mu }}\text{+}{}^{12}\text{B}$ reaction. We obtain also dynamical information on μ-capture: (i) the weak magnetism form factor, μ=4.5±1.1, and (ii) the sum of the induced pseudoscalar (g_p) and the 2nd class induced tensor (g_T) couplings versus g_A, ($\text{g}{}_{\mathrm{<mtext>P</mtext>}}\text{+g}{}_{\mathrm{<mtext>T</mtext>}}\text{)}\text{g}{}_{\mathrm{<mtext>A</mtext>}}\text{=7.1±2.7}$. The latter result, adopting the “canonical” value of $\text{g}{}_{\mathrm{<mtext>P</mtext>}}\text{g}{}_{\mathrm{<mtext>A</mtext>}}$, leads to $\text{g}{}_{\mathrm{<mtext>T</mtext>}}\text{g}{}_{\mathrm{<mtext>A</mtext>}}\text{=+1±2.7}$ which is compatible with zero and in strong contradiction with the value ?—6 recently advocated by Kubodera, Delorme and Rho.