Electric field effects on an optically-pumped HCOOH FIR laser and Zeeman laser theory

Electric field effects have been investigated on the output power of six far-infrared (FIR) laser lines from H¹²COOH optically-pumped by a CO₂ laser with its polarization arranged perpendicular to the Stark field. Optoacoustic signals observed on the pump lines were hardly affected by the applied electric field up to 0.6 kV/cm. By neglecting the electric field effects on the pump transitions, Zeeman laser theory has been applied to the FIR laser transitions. Numerical calculation predicts the observed FIR output power as a function of electric field. Experessions for oscillation frequency and intensity in homogeneous limit are given, which may be applicable to any FIR Stark laser so far as the pump transition is free from electric field effects.     

Effects of Buffer Gas on the Output of Optically Pumped NH3 Far-Infrared Cavity Laser

By solving the semi-classical density matrix equations and developing a buffer gas mechanism model, the effects of buffer gas on the output power of optically pumped NH₃ far-infrared cavity laser were calculated and verified by experiment. Our results showed that: the output power of NH₃ far-infrared laser could be increased when certain buffer gas was added into the laser medium, and there existed an optimum ratio of gases mixture and an optimum operating gas pressure which could make the output power of far-infrared laser reach maximum.     

New Far-Infrared Laser Lines and Frequency Measurements of Acetaldehyde and Vinyl Fluoride

Eight far-infrared laser lines have been obtained by optically pumping acetaldehyde (CH₃CHO) and nine by pumping vinyl fluoride (CH₂CHF) with a cw CO₂ laser. The far-infrared laser structure used a metal-dielectric waveguide cavity. This is the first reported observation of four of the laser lines in acetaldehyde. In this work, we measure the frequency, optimum pressure of operation, relative intensity, relative polarization, and pump offset from CO₂ laser-line center.     

Investigation for long wavelength fir laser lines for EPR studies: New lines from CH2=CF2

The results described in this work are part of a systematic search for long wavelength laser lines to be used in high magnetic field EPR applications and in plasma diagnostic. Four new far-infrared laser lines of CH₂ = CF₂ (1,1 difluoroethylene), optically pumped by a waveguide CO₂ laser, have been discovered and characterized in wavelength, polarization relative to the pumping radiation and offset relative to the CO₂ center frequency. New measurements of polarization and offset of 5 already known laser lines are also reported. A table of all of the known CO₂ pumped FIR laser lines from this molecule is given.     

Assignment of Fir Laser Lines of Fully Deuterated Dichloromethane

We have recently reported 16 new far-infrared laser emissions of CD₂Cl₂. While the overwhelming majority of the previously known FIR laser emissions of this molecule were polarized parallel to the polarization of the pump CO₂ line, 13 of our 16 new lines are polarized perpendicularly to the exciting CO₂ radiation. In principle, the presence of perpendicular/parallel emission pairs is extremely important for the assignment of laser transitions. In the present work we discuss the possible assignments of 16 far-infrared (FIR) laser emission pairs of CD₂Cl₂.     

New far-infrared emissions and frequency measurements in hydrazine

By means of a new CO₂ laser we performed a new investigation of the far-infrared laser emission spectrum of hydrazine excited by the 10P(32) and 10R(8) CO₂ laser lines. We found seven new lines and measured the frequency of four of them; moreover we measured the frequencies of two more lines previously reported in the literature with only wavelength measurements. The frequencies of the far-infrared laser emissions have been measured by means of a frequency-synthesis chain based on new InP Schottky diodes. The detected signal was beat-note generated in a Schottky diode between the far-infrared radiation, the harmonics of a 72 GHz frequency reference and a rf signal. We also characterized all of the observed lines by their polarization relative to the pumping CO₂ laser, the optimum pressure and the offset relative to the CO₂ center frequency. PACS 42.55.Lt; 42.62.Fi     

12CH3OH and 13CH3OH optically pumped by the 10P and 10HP bands of a pulsed CO2 laser: New far-infrared laser emissions and assignments

We have re-investigated the ¹²CH₃OH and the ¹³CH₃OH molecules as optically pumped far-infrared laser sources. We have used our new waveguide pulsed-high-peak-power CO₂ laser for pumping, finding 20 new far-infrared laser lines emitted by ¹²CH₃OH and seven emitted by ¹³CH₃OH. For each line we report wavelength, pump offset from the center of the exciting CO₂ line, relative polarization, optimum operating pressure and intensity. The LaseRitz program was able to assign one of the new laser systems of ¹²CH₃OH, involving two new far-infrared laser lines.PACS 42.55.Lt; 42.62.Fi     

远红外固体激光器研究进展

8～12μm波段是大气的一个窗口,被定义为长波红外波段。该波段激光对雾、烟尘等具有较强的穿透力,在激光光电对抗、激光遥感、医疗、环境监测及光通讯领域具有重要的应用前景。本文调研了常用的8～12μm非线性频率变换晶体,以及基于非线性频率变换晶体的远红外光参量振荡器的研究进展,对国内外能实现8～12μm波段激光输出的非线性晶体及激光系统进行了系统地归纳和总结,通过分析比较得出在8～12μm波段获得的最大输出能量为毫焦量级,最大功率为瓦量级。国内该技术与国外有着不小的差距,主要受制于高重频、高功率脉冲1～3μm泵浦源技术不成熟及高性能非线性晶体材料研制基础薄弱,我国在长波远红外固体激光器领域研究进展缓慢,因此研制大尺寸、高质量远红外激光晶体及输出波长更长的远红外高功率激光器已经成为激光器未来发展方向之一。     

Spectra of optically pumped superradiant and cavity NH3 far-infrared laser

Based on the density matrix theory of quantum system, the spectra of optically pumped superradiant and cavity NH₃ far-infrared (FIR) lasers were calculated by means of iteration method. The calculation showed that, compared with the optically pumped superradiant FIR laser, the cavity laser had a wider band spectrum of FIR emission and a higher output power under certain condition, moreover, the spectra of cavity laser had multi longitudinal-mode structure. Supported by the Research Foundation of Hubei Province Education Committee, PRC     

A magneto-optically modulated CH3OH laser for Faraday rotation measurements in Tokamaks

Distortion-free intracavity polarization modulation of an optically pumped CH₃OH laser is shown to be viable. The possible use of this modulation technique to make a multichannel Faraday rotation measurement on a Tokamak device is discussed. In addition, the CdTe Faraday modulator employed in this study is shown to have an anomalously large Verdet constant.     

Relaxation oscillations in cw optically pumped CD3OD and15NH3 lasers

We report the results of heterodyne measurements of the mode quality and tuning range of a cw CO₂ laser designed for optically pumping a far-infrared (FIR) molecular laser, and describe the implications of multi-mode operation. In particular we report the observation of relaxation oscillations in the output of a FIR waveguide laser.     

New FIR Laser Lines from CHD2OH Methanol

We have investigated CHD₂OH methanol as source of far-infrared (FIR) laser radiation using the optical pumping technique. Our new waveguide pulsed CO₂ laser, with peak powers as high as some kW, has allowed us to observe 12 new lines. Each of them is characterized in wavelength, relative polarization, intensity, optimum operating pressure and pump offset from the center of the exciting CO₂ line.     

New FIR laser lines from hydrazine and assignments

Our new waveguide pulsed CO₂ laser, with peak powers above 1 kW, has allowed us to observe 24 new far-infrared laser lines emitted by hydrazine. Each of them is characterized in wavelength, relative polarization, intensity, optimum operating pressure and pump offset from the center of the exciting CO₂ line. These new laser emissions either form pairs sharing the same pump line, or complete such pairs with lines known from the literature. In the latter case, we have measured the relative polarization and offset of the partner lines whenever they were not reported in the literature. The availability of laser systems with two emission lines orthogonally polarized and sharing the same upper level is expected to facilitate the assignment work. We present complete assignments for four FIR laser emissions, and we propose J and K values for 12 further laser systems. PACS 42.55.Lt; 42.62.Fi     

Laser frequency measurements and spectroscopic assignments of optically pumped 13CH3OH

A three-laser heterodyne system was used to measure the frequencies of twelve optically pumped laser emissions from ¹³CH₃OH in the far-infrared (FIR) region. These emissions, ranging from 54 to 142 μm, are reported with fractional uncertainties up to ±2×10^-7 along with their polarization relative to the CO₂ pump. Using the 9P32 and 10R14 CO₂ lines, complete spectroscopic assignments for two laser systems were confirmed. Received: 31 May 2001 / Published online: 19 September 2001     

Smith–Purcell free electron laser based on a semi-conical resonator

We investigate a Smith–Purcell free electron laser composed of an electron gun, a semi-conical resonator, a metallic grating and collector. The semi-conical resonator could reflect all Smith–Purcell radiation with emission angle θ, and with random azimuthal angles, back onto the electron beam and causes the electrons to be modulated. Tunable coherent far-infrared Smith–Purcell radiation with a high output peak power at millimeter wavelengths can be generated.     

Study of laser output power stabilization for a deuterium cyanide laser interferometer on the Experimental Advanced Superconducting Tokamak

A control system which can improve stabilization of laser power in long-term operation automatically is designed for a deuterium cyanide (DCN) far-infrared laser interferometer on the Experimental Advanced Superconducting Tokamak. It stabilizes the output power of the laser by a closed-loop control system aided by a programmable logic controller. The system has been applied to the DCN laser and it has been proven that it is effective in stabilizing the laser near the highest scope of the output power.     

The Optimum Coupling Coefficient of Optically Pumped NH3 Far-Infrared Cavity Laser

Based on the semiclassical density matrix theory, the optimum output power reflection coefficient (coupling coefficient) of output coupler for optically pumped NH₃ far-infrared (FIR) cavity laser was calculated by means of iteration method. Experimentally, FIR Fabry-Perot cavity laser was designed and constructed by using inductive metallic meshes as couplers, and the measurement showed that the theoretical calculation were in agreement with experimental results.     

高气压TE CO2激光泵浦的高功率连续可调谐远红外喇曼NH3激光器

本文报道输出能量约4mJ(功率约80kW)的连续可调谐远红外喇曼跃迁NH₃激光器,调谐范围约覆盖发射谱从90到93μm的70％。分立K能级激光跃迁的连续调谐范围约为30GHz。文中给出了典型的实验结果,并进行了讨论。 关键词：     

Infrared and far-infrared spectroscopy of CH3OH: TeraHertz laser lines and assignments

We use a ¹³CO₂ laser as optical pumping source to search for new THz laser lines generated from ¹³CH₃OH. Nineteen new THz laser lines (also identified as far-infrared, FIR) ranging from 42.3 μm (7.1 THz) to 717.7 μm (0.42 THz) are reported. They are characterized in wavelength, offset, relative polarization, relative intensity, and optimum working pressure. We have assigned eight laser lines to specific rotational energy levels in the excited state associated with the C-O stretching mode.     

Comparison of laser performance of Yb:YCa4O(BO3)3 crystals cut along the principal optical axes

Efficient high-power continuous-wave laser operation is demonstrated with Yb:YCa₄O(BO₃)₃ crystals cut along the X, Y, and Z principal axes, end pumped by a high-power diode. Highest output powers of 6.3–7.3 W are generated, with slope efficiencies in the range of 73–83%. The standard behavior characterized by fixed linear polarization of the output and decreasing oscillation wavelength when increasing the output coupling was observed only for the X-cut crystal; the Y-cut crystal led to the polarization state changing and coexistence, while the Z-cut crystal resulted in dual-band laser operation with a fixed polarization state. PACS 42.55.Rz; 42.55.Xi