高等学校化学学报 ›› 2019, Vol. 40 ›› Issue (5): 855.doi: 10.7503/cjcu20180688
何鹏琛, 周健, 周阿武, 豆义波(
), 李建荣()
收稿日期:2018-10-15
出版日期:2019-05-06
发布日期:2019-07-04
作者简介:联系人简介: 豆义波, 男, 博士, 副研究员, 主要从事金属有机框架基复合功能材料研究. E-mail:
基金资助:
HE Pengchen, ZHOU Jian, ZHOU Awu, DOU Yibo*(), LI Jianrong*()
Received:2018-10-15
Online:2019-05-06
Published:2019-07-04
Contact:
DOU Yibo,LI Jianrong
E-mail:douyb@bjut.edu.cn;jrli@bjut.edu.cn
Supported by:摘要：
系统总结了金属有机框架(MOFs)基材料在光催化还原CO2中的最新研究进展, 其中包括MOFs直接作为光催化剂和作为复合光催化2个主要部分, 讨论了MOFs基光催化剂在催化还原CO2方面展现出的独特优势, 并对MOFs基光催化剂的结构稳定性与CO2转化效率等问题进行讨论与分析, 对未来发展趋势进行了展望.
中图分类号:
TrendMD:
何鹏琛, 周健, 周阿武, 豆义波, 李建荣. MOFs基材料在光催化CO2还原中的应用. 高等学校化学学报, 2019, 40(5): 855.
HE Pengchen,ZHOU Jian,ZHOU Awu,DOU Yibo,LI Jianrong. MOFs-Based Materials for Photocatalytic CO2 Reduction†. Chem. J. Chinese Universities, 2019, 40(5): 855.
Fig.1 Structure(A) and CO2 and N2 adsorption isotherms(B) of PCN-222, UV-Vis spectra of PCN-22 and H2TCPP(C) and the amount of HCOO-(D) with PCN-22 as catalyst[33] (D) a. PCN-222; b H2TCPP; c. no PCN-222; d. no TEOA; e. no CO2. Copyright 2015, American Chemical Society.
Fig.2 Ligand structure of H2L1-H2L6(A), photocatalytic conversion schematic(B), plots of CO-TON versus time(C) and PXRD patterns of the catalysts(D)[41] Copyright 2011, American Chemical Society.
Fig.3 Structures of Ren-MOF and Ag?Ren-MOF based catalysts(A), PXRD of Ren-MOFs(B) and the photocatalytic activity of Ren-MOF(C)[42] Copyright 2017, American Chemical Society.
Fig.4 XRD patterns(A) and FTIR spectra(B), N2(C) and CO2(D) adsorption and desorption isotherms of SCu and SP[43] Copyright 2013, American Chemical Society.
Fig.5 Fabrication of Cu-TiO2/ZIF-8 membranes(A), effect of membrane composition(B) and Cu-TiO2 nanoparticles loading on the product yields(C)[51] Copyright 2017, American Chemical Society.
Fig.6 HKUST-1 and HKUST-1/TiO2 formation steps inside a microdroplet(A), TEM images of as-synthesized HKUST-1(B) and 33.3 HKUST-1/TiO2(C) at 300 ℃ and CO2 photoreduction performance of TiO2 and HKUST-1/TiO2 composites(D)[52] Inset of (B): the image of the contact angle measurement of HKUST-1 surface. Copyright 2017, American Chemical Society.
Fig.7 Schematic illustration of the fabrication process and CO2 photoreduction process of CsPbBr3/ZIFs(A) and photocatalytic CO2 reduction performances of CsPbBr3 and CsPbBr3@ZIFs(B, C)[59] Copyright 2018, American Chemical Society.
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