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Three‐Dimensional Ordered Assembly of Thin‐Shell Au/TiO2 Hollow Nanospheres for Enhanced Visible‐Light‐Driven Photocatalysis
Authors:Cao‐Thang Dinh  Hoang Yen  Prof. Freddy Kleitz  Prof. Trong‐On Do
Affiliation:1. Department of Chemical Engineering and Centre de recherche sur les propriétés des interfaces et la catalyse (CERPIC), Université Laval, Quebec, G1V 0A6 (Canada);2. Department of Chemistry and Centre de recherche sur les matériaux avancés (CERMA), Université Laval, Quebec, G1V 0A6 (Canada)
Abstract:An Au/TiO2 nanostructure was constructed to obtain a highly efficient visible‐light‐driven photocatalyst. The design was based on a three‐dimensional ordered assembly of thin‐shell Au/TiO2 hollow nanospheres (Au/TiO2‐3 DHNSs). The designed photocatalysts exhibit not only a very high surface area but also photonic behavior and multiple light scattering, which significantly enhances visible‐light absorption. Thus Au/TiO2‐3 DHNSs exhibit a visible‐light‐driven photocatalytic activity that is several times higher than conventional Au/TiO2 nanopowders.
Keywords:gold  nanostructures  ordered assembly  photocatalysis  titanium dioxide
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