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层状双金属氧化物材料对放射性核素的去除研究
引用本文:王祥学,庞宏伟,吴忆涵,于淑君,宋刚,马宵颖,许佩瑶.层状双金属氧化物材料对放射性核素的去除研究[J].中国科学:化学,2019(1):2-11.
作者姓名:王祥学  庞宏伟  吴忆涵  于淑君  宋刚  马宵颖  许佩瑶
作者单位:华北电力大学环境科学与工程系;华北电力大学环境科学与工程学院;广东省放射性核素污染控制与资源化重点实验室
基金项目:中央高校基本科研业务费专项资金(编号:2018MS114;2018ZD11);广东省放射性核素污染控制与资源化重点实验室开放基金(编号:GZDX2017K001)资助项目
摘    要:层状双金属氧化物材料(LDHs)作为最常见的二维材料,在环境污染治理领域展现出巨大的优势. LDHs具有来源广泛、易于制备、较大的表面积、可调控的化学结构、环境友好等优点,最近几年其改性材料多用于放射性核素的高效去除.本文介绍了常用的LDHs材料及其衍生物的制备方法以及它们在放射性核素处理方面的应用及其相互作用机制,最后对LDHs材料的应用和挑战给出了个人见解.本综述为高效去除放射性核素的LDHs材料的设计指明了方向,为放射性核素的高效处理处置提供了新材料.

关 键 词:双金属氧化物材料  放射性核素  吸附  分析表征  作用机理

Removal of radionuclides by layered double hydroxides materials
Xiangxue Wang,Hongwei Pang,Yihan Wu,Shujun Yu,Gang Song,Xiaoying Ma,Peiyao Xu.Removal of radionuclides by layered double hydroxides materials[J].Scientia Sinica Chimica,2019(1):2-11.
Authors:Xiangxue Wang  Hongwei Pang  Yihan Wu  Shujun Yu  Gang Song  Xiaoying Ma  Peiyao Xu
Institution:(Department of Environmental Science and Engineering,North China Electric Power University,Baoding 071003,China;College of Environmental Science and Engineering,North China Electric Power University,Beijing 102206,China;Guangdong Provincial Key Laboratory of Radionuclides Pollution Control and Resources,Guangzhou 510006,China)
Abstract:Layered double hydroxides(LDHs),one of the most important two-dimensional layered compounds,have enabled massive developments in effective pollution treatments.Over the past few decades,their derivative materials have also applied to the efficient removal of radionuclides owing to the intrinsic advantages of their low cost,easy preparation,large surface areas,topological transformation,and environment-friendly.In this review,we give an overview of the recent advances in LDH-based nanomaterials,from a brief introduction to their preparation and modification methods to an overview of their application in the removal of radionuclides and an exploration of their underlying adsorption mechanisms.In the end,a summary and outlook are also briefly addressed.This review intends to provide deep insight into the design of high-performance LDH-based materials for the potential elimination of radionuclides from aqueous solutions during environmental pollution cleanup.
Keywords:layered double hydroxides(LDHs)  radionuclides  adsorption  analytical characterization  interaction mechanism
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