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Recent progress in advanced core-shell metal-based catalysts for electrochemical carbon dioxide reduction
作者姓名:Fengqi Wang  Wenlong Zhang  Hongbin Wan  Chenxi Li  Wankai An  Xia Sheng  Xiaoyu Liang  Xiaopeng Wang  Yunlai Ren  Xin Zheng  Dongcan Lv  Yuchen Qin
作者单位:1. College of Sciences, Henan Agricultural University;2. Oilfield Technology Research Institute of Fengcheng Oilfield Operation Area,Xinjiang Oilfield Company;3. College of Life Science, Chongqing Normal University
基金项目:funded by the National Natural Science Foundation of China (Nos. 21706074 and 21972038);;the Natural Science Foundation of Henan Province (No. 2023000410209);;The Science and Technology Research Program of Chongqing Municipal Education Commission (No. KJQN202000519);
摘    要:Electrochemical carbon dioxide reduction(CO2RR) plays an important role in solving the problem of high concentration of CO2in the atmosphere and realizing carbon cycle. Core-shell structure has many unique features including tandem catalysis, lattice strain effect, defect engineering, which exhibit great potential in electrocatalysis. In this review, we focus on the advanced core-shell metal-based catalysts(CMCs) for electrochemical CO2RR. The recent progress of ...

收稿时间:14 June 2021

Recent progress in advanced core-shell metal-based catalysts for electrochemical carbon dioxide reduction
Fengqi Wang,Wenlong Zhang,Hongbin Wan,Chenxi Li,Wankai An,Xia Sheng,Xiaoyu Liang,Xiaopeng Wang,Yunlai Ren,Xin Zheng,Dongcan Lv,Yuchen Qin.Recent progress in advanced core-shell metal-based catalysts for electrochemical carbon dioxide reduction[J].Chinese Chemical Letters,2022,33(5):2259-2269.
Institution:1. College of Sciences, Henan Agricultural University, Zhengzhou 450000, China;2. Oilfield Technology Research Institute of Fengcheng Oilfield Operation Area, Xinjiang Oilfield Company, Karamay 834000, China;3. College of Life Science, Chongqing Normal University, Chongqing 401331, China
Abstract:Electrochemical carbon dioxide reduction (CO2RR) plays an important role in solving the problem of high concentration of CO2 in the atmosphere and realizing carbon cycle. Core-shell structure has many unique features including tandem catalysis, lattice strain effect, defect engineering, which exhibit great potential in electrocatalysis. In this review, we focus on the advanced core-shell metal-based catalysts (CMCs) for electrochemical CO2RR. The recent progress of CMCs in electrocatalytic CO2RR is described as the following aspects: (1) The mechanism of electrochemical CO2RR and evaluation parameters of electrocatalyst performance, (2) preparation methods of core-shell metal catalysts and core-shell structural advantages and (3) advanced CMCs towards electrochemical CO2RR. Finally, we make a brief conclusion and propose the opportunities and challenges in the field of electrochemical CO2RR.
Keywords:
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