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CoFe-LDH nanowire arrays on graphite felt: A high-performance oxygen evolution electrocatalyst in alkaline media
Authors:Biao Deng  Jie Liang  Luchao Yue  Tingshuai Li  Qian Liu  Yang Liu  Shuyan Gao  Abdulmohsen Ali Alshehri  Khalid Ahmed Alzahrani  Yonglan Luo  Xuping Sun
Institution:1. Chemical Synthesis and Pollution Control Key Laboratory of Sichuan Province, School of Chemistry and Chemical Engineering, China West Normal University, Nanchong 637002, China;2. Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu 610054, China;3. Institute for Advanced Study, Chengdu University, Chengdu 610106, China;4. School of Materials Science and Engineering, Henan Normal University, Xinxiang 453007, China;5. Chemistry Department, Faculty of Science, King Abdulaziz University, P.O. Box 80203, Jeddah 21589, Saudi Arabia
Abstract:Developing non-noble-metal oxygen evolution reaction (OER) electrocatalysts with high performance is critical to electrocatalytic water splitting. In this work, we fabricated CoFe-layered double hydroxide (LDH) nanowire arrays on graphite felt (CoFe-LDH/GF) via a hydrothermal method. The CoFe-LDH/GF, as a robust integrated 3D OER anode, exhibits excellent catalytic activity with the need of low overpotential of 252 and 285 mV to drive current densities of 10 and 100 mA/cm2 in 1.0 mol/L KOH, respectively. In addition, it also maintains electrochemical durability for at least 24 h. This work would open up avenues for the development of GF like attractive catalyst supports for oxygen evolution applications.
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