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Developments on carbon dioxide reduction: Their promise,achievements, and challenges
Authors:Samuel C Perry  Pui-ki Leung  Ling Wang  Carlos Ponce de León
Institution:1. Electrochemical Engineering Laboratory, Energy Technology Research Group, Faculty of Engineering and Physical Sciences, University of Southampton, Highfield, Southampton, SO17 1BJ, UK;2. National Centre of Advanced Tribology at Southampton (NCATS), Faculty of Engineering and Physical Sciences, University of Southampton, University Rd., Southampton, SO17 1BJ, UK
Abstract:CO2 reduction processes continue to be developed for electrosynthesis, energy storage applications, and environmental remediation. A number of promising materials have shown high activity and selectivity to target reduction products. However, the progress has been mainly at a small laboratory scale, and the technical challenges of large scale CO2 reduction have not been considered adequately. This review covers recent advancements in catalyst materials and cell designs. The leading materials for CO2 reduction to a number of useful products are presented with their corresponding cell and reactor designs. The latest efforts to progress to industrially relevant scales are discussed, along with the challenges that must be met for carbon dioxide reduction to be a viable route for mass scale production.
Keywords:Carbon dioxide reduction  Electrosynthesis  Energy storage  carbon dioxide reduction reaction  HER"}  {"#name":"keyword"  "$":{"id":"kwrd0040"}  "$$":[{"#name":"text"  "_":"hydrogen evolution reaction  FE"}  {"#name":"keyword"  "$":{"id":"kwrd0050"}  "$$":[{"#name":"text"  "_":"Faradaic efficiency  GDE"}  {"#name":"keyword"  "$":{"id":"kwrd0060"}  "$$":[{"#name":"text"  "_":"gas diffusion electrode  MEA"}  {"#name":"keyword"  "$":{"id":"kwrd0070"}  "$$":[{"#name":"text"  "_":"membrane electrode assembly  PEM"}  {"#name":"keyword"  "$":{"id":"kwrd0080"}  "$$":[{"#name":"text"  "_":"proton exchange membrane  SEM"}  {"#name":"keyword"  "$":{"id":"kwrd0090"}  "$$":[{"#name":"text"  "_":"scanning electron microscope
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