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STUDY OF THE CATALYTIC TECHNOLOGY IN THE OXIDATIVE COUPLING OF METHANE
作者姓名:XIE Mao-Song WANG Xue-Lin XU Gui-Fen WANG Lin-Shang TAO Long-XiangDalian Institute of Chemical Physics  Academia Sinaca Datum  Liaomig
作者单位:XIE Mao-Song WANG Xue-Lin XU Gui-Fen WANG Lin-Shang TAO Long-XiangDalian Institute of Chemical Physics,Academia Sinaca Datum,Liaomig 116023
摘    要:The temperature of the catalyst bed in the oxidative coupling ofmethane would rise and be higher than the wall temperature when the amountof catalyst, the space velocity and the ratio of oxygen to methane wereincreased. Various aspects of the catalytic technology including the thickness ofthe catalyst bed, the mode of catalyst charge, the ratio of CH_4 to O_2 and thespece velocity were studied. An optimum temperature of the catalyst bed forhigher methane conversion and C_2 selectivity was investigated. It was foundthat the burning of methane in the gas phase to form CO occurred at certaintemperatures with some ratios of oxygen to methane. Additionally, the effectof adding water to the reaction feed gas was studied.


STUDY OF THE CATALYTIC TECHNOLOGY IN THE OXIDATIVE COUPLING OF METHANE
XIE Mao-Song WANG Xue-Lin XU Gui-Fen WANG Lin-Shang TAO Long-XiangDalian Institute of Chemical Physics,Academia Sinaca Datum,Liaomig .STUDY OF THE CATALYTIC TECHNOLOGY IN THE OXIDATIVE COUPLING OF METHANE[J].Journal of Natural Gas Chemistry,1995(2).
Authors:XIE Mao-Song WANG Xue-Lin XU Gui-Fen WANG Lin-Shang TAO Long-XiangDalian Institute of Chemical Physics  Academia Sinaca Datum  Liaomig
Institution:XIE Mao-Song WANG Xue-Lin XU Gui-Fen WANG Lin-Shang TAO Long-XiangDalian Institute of Chemical Physics,Academia Sinaca Datum,Liaomig 116023
Abstract:The temperature of the catalyst bed in the oxidative coupling of methane would rise and be higher than the wall temperature when the amount of catalyst, the space velocity and the ratio of oxygen to methane were increased. Various aspects of the catalytic technology including the thickness of the catalyst bed, the mode of catalyst charge, the ratio of CH4 to O2and the space velocity were studied. An optimum temperature of the catalyst bed for higher methane conversion and C2 selectivity was investigated. It was found that the burning of methane in the gas phase to form CO occurred at certain temperatures with some ratios of oxygen to methane. Additionally, the effect of adding water to the reaction feed gas was studied.
Keywords:methane  oxidative coupling  catalytic technology
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