CH(4) storage and CO(2) capture in highly porous zirconium oxide based metal-organic frameworks |
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| Authors: | Qingyuan Yang Vincent Guillerm Florence Ragon Andrew D Wiersum Philip L Llewellyn Chongli Zhong Thomas Devic Christian Serre Guillaume Maurin |
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| Institution: | State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing 100029, China. |
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| Abstract: | A series of porous Zr oxoclusters-based MOFs was computationally explored for their gas storage/capture performances. The highly porous UiO-67(Zr) and UiO-68(Zr) solids show exceptionally high CH(4) and CO(2) adsorption capacities under operating conditions that make these thermal, water and mechanical resistant materials very promising for physisorption-based processes. |
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