Photoinduced Polaron-Splitting in Polymer |
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作者姓名: | 唐菲 徐晓华 孙鑫 |
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作者单位: | [1]ResearchCentreforTheoreticalPhysics,FudanUniversity,Shanghai200433 [2]NationalLaboratoryofInfraredPhysics,ShanghaiInstituteofTechnicalPhysics,ChineseAcademyofSciences,Shanghai200083 |
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摘 要: | We simulate a relaxation process of a polaron in polymer after photo excitation, and a new state is realized by means of proper excitation. The original lattice configuration of the polaron splits into two symmetrical peaks, and consequently a double-well potential is formed, where the wavefunctions of electron localized in these two wells are entangled. Thus, this process provides a method to generate the Schroedinger cat state. According to the dynamical process of the lattice configuration, the relaxation time of splitting is about 150fs.
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关 键 词: | 聚合物 极化子 光诱导 波函数 薛定谔猫态 哈密顿算法 |
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