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Ultrafast carrier dynamics in purified and as-grown single-walled carbon nanotube films
作者姓名:龙拥兵  宋礼  张春雨  汪力  傅盘铭  张治国  解思深  汪国平
作者单位:Department of Physics, Wuhan University, Wuhan 430072, China;Laboratory of Optical Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100080, China;Center for Condensed Matter Physics, Institute of Physics,Chinese Academy of Sciences, Beijing 100080, China;Laboratory of Optical Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100080, China;Laboratory of Optical Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100080, China;Laboratory of Optical Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100080, China;Laboratory of Optical Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100080, China;Center for Condensed Matter Physics, Institute of Physics,Chinese Academy of Sciences, Beijing 100080, China;Department of Physics, Wuhan University, Wuhan 430072, China
基金项目:Project supported by the Laboratory of Optical Physics, Institute of Physics, Chinese Academy of Sciences.
摘    要:Ultrafast time-resolved optical transmissions in purified and as-grown single-walled carbon nanotube films are measured at a temperature of 200K. The signal of the purified sample shows a crossover from photobleaching to photoabsorption. The former and the latter are interpreted as the state filling and the red shift of the π-plasmon, respectively. The signal of the as-grown sample can be perfectly fitted by a single-exponential with a time constant of 232fs. The disappearance of the negative component in the as-grown sample is attributed to the charge transfer between the semiconducting nanotubes and the impurities.

关 键 词:carbon  nanotubes    carrier  dynamics    ∏-plasmon  resonance    charge  transfer
收稿时间:2/3/2005 12:00:00 AM
修稿时间:2005-02-032005-06-16

Ultrafast carrier dynamics in purified and as-grown single-walled carbon nanotube films
Long Yong-Bing,Song Li,Zhang Chun-Yu,Wang Li,Fu Pan-Ming,Zhang Zhi-Guo,Xie Si-Shen and Wang Guo-Ping.Ultrafast carrier dynamics in purified and as-grown single-walled carbon nanotube films[J].Chinese Physics B,2005,14(10):2137-2140.
Authors:Long Yong-Bing  Song Li  Zhang Chun-Yu  Wang Li  Fu Pan-Ming  Zhang Zhi-Guo  Xie Si-Shen and Wang Guo-Ping
Institution:Center for Condensed Matter Physics, Institute of Physics,Chinese Academy of Sciences, Beijing 100080, China; Department of Physics, Wuhan University, Wuhan 430072, China; Department of Physics, Wuhan University, Wuhan 430072, China;Laboratory of Optical Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100080, China; Laboratory of Optical Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100080, China
Abstract:Ultrafast time-resolved optical transmissions in purified and as-grown single-walled carbon nanotube films are measured at a temperature of 200K.The signal of the purified sample shows a crossover from photobleaching to photoabsorption. The former and the latter are interpreted as the state filling and the red shift of the $\pi$-plasmon, respectively. The signal of the as-grown sample can be perfectly fitted by a single-exponential with a time constant of 232fs. The disappearance of the negative component in the as-grown sample is attributed to the charge transfer between the semiconducting nanotubes and the impurities.
Keywords:carbon nanotubes  carrier dynamics  zr-plasmon resonance  charge transfer
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