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C60醛类衍生物非线性光学特性研究
引用本文:王沛,张为俊,程平,葛传文,聂劲松,唐晓加,杨顒,魏先文,徐正.C60醛类衍生物非线性光学特性研究[J].光学学报,2001,21(2):22-224.
作者姓名:王沛  张为俊  程平  葛传文  聂劲松  唐晓加  杨顒  魏先文  徐正
作者单位:1. 中国科学院安徽光学精密机械研究所
2. 南京大学配位化学研究所,
摘    要:研究了加合不同取代基团的C60醛类衍生物的光学非线性性质。利用简并四波混频(DFMW)方法获得了C60醛类各衍生物的三阶光学非线性超级化率γ^(3)及相应的三阶光学非线性系数χ^(3)值。同时也研究了它们各自的光限幅特性。结果表明:不同的取代基对C60醛类衍生物三阶光学非线性及光限幅特性的影响不同。

关 键 词:取代基团  碳60  醛类衍生物  三阶光学非线性  光限幅特性  简并四波混频

Nonlinear Optical Properties of C60 Derivatives
Wang Pei,Zhang Weijun,Cheng Ping,Ge Chuanwen,Nie Jinsong,Tang Xiaojia,Yang Yong,WEI Xianwen,Xu Zheng.Nonlinear Optical Properties of C60 Derivatives[J].Acta Optica Sinica,2001,21(2):22-224.
Authors:Wang Pei  Zhang Weijun  Cheng Ping  Ge Chuanwen  Nie Jinsong  Tang Xiaojia  Yang Yong  WEI Xianwen  Xu Zheng
Abstract:The nonlinear optical properties of a series of C60 derivatives with different substituents are reported. The optical limiting properties were measured using the second harmonic of a Q-switched Nd∶YAG at 532 nm, the third-order optical nonlinearities of C60 derivatives in solution were studied by nanosecond degenerate four-wave-mixing(DFWM) experiment. The values of the third-order hyperpolarizabilities γ(3) and the third-order nonlinear optical susceptibilities χ(3) of C60 derivatives were obtained, respectively. Experimental results show that different substituents have different effects on the nonlinear optical properties of C60 derivatives.
Keywords:substituent  C    60  derivatives  nonlinear optical property
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