Observation of a new coherent transient in NMR -- nutational two-pulse stimulated echo in the angular distribution of \gamma-radiation from oriented nuclei |
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Authors: | LN Shakhmuratova WD Hutchison DJ Isbister DH Chaplin |
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Institution: | (1) School of Physics, University College, The University of New South Wales, Australian Defence Force Academy, Canberra, ACT, 2600, Australia |
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Abstract: | A new coherent transient in pulsed NMR, the two-pulse nutational stimulated echo, is reported for the ferromagnetic system
60CoFe using resonant perturbations on the directional emission of anisotropic \gamma-radiation from thermally oriented nuclei.
The new spin echo is a result of non-linear nuclear spin dynamics due to large Larmor inhomogeneity active during radiofrequency
pulse application. It is made readily observable through the gross detuning between NMR radiofrequency excitation and gamma
radiation detection, and inhomogeneity in the Rabi frequency caused by metallic skin-effect. The method of concatenation of
perturbation factors in a statistical tensor formalism is quantitatively applied to successfully predict and then fit in detail
the experimental time-domain data.
This revised version was published online in August 2006 with corrections to the Cover Date. |
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