Linear and nonlinear optical properties of ZnO nanorod arrays |
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Authors: | Xiao Si Su Xiong-Rui Li Chun Han Yi-Bo Fang Guo-Jia and Wang Qu-Quan |
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Institution: | Department of Physics, Wuhan University, Wuhan
430072, China; Department of Physics, Wuhan University, Wuhan
430072, China;Key Laboratory of Acoustic and Photonic Materials and
Devices of Ministry of Education,
Wuhan University, Wuhan
430072, China |
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Abstract: | Polarization-dependent linear absorption, second-harmonic generation
(SHG) and 3rd-order nonlinearities of well-aligned ZnO nanorod
arrays have been investigated with ps pulses. The depressed spectral
width and the enhanced intensity of reflective SHG along the long
axis of ZnO nanorods were observed by using p-polarized pulses,
which is explained by the optical confinements. The nonlinear
absorption coefficient measured with s-polarization reached the
maximum 4.0$\times $10$^{4}$cm/GW at the wavelength $\sim $750\,nm,
which revealed a large two-photon resonance absorption attributed to
the quantum confined exciton when the polarization is vertical to
the long axis of ZnO nanorod. |
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Keywords: | ZnO nanorods second-harmonic
generation nonlinearity |
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