Interference of dissociating wave packets in the I2 molecule driven by femtosecond laser pulses |
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Authors: | Han Yong-Chang Hu Wen-Hui Yu Jie and Cong Shu-Lin |
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Institution: | Department of Physics, Dalian University of Technology, Dalian
116024, China |
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Abstract: | The interference between two dissociating wave packets of
the \textrmI2 molecule driven by femtosecond laser pulses is
theoretically studied by using the time-dependent quantum wave packet
method. Both the internuclear distance- and velocity-dependent
density functions are calculated and discussed. It is demonstrated
that the interference pattern is determined by the phase difference
and the delay time between two pump pulses. With two identical
pulses with a delay time of 305~fs and a FWHM of 20~fs, more
interference fringes can be observed, while with two pump pulses
with a delay time of 80~fs and a FWHM of 20~fs, only a few
interference fringes can be observed. |
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Keywords: | photodissociation interference of wave packets I2
molecule |
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