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Generation of an isolated sub-100 attosecond pulse in the water-window spectral region
Authors:Zou Pu  Li Ru-Xin  Zeng Zhi-Nan  Xiong Hui  Liu Peng  Leng Yu-Xin  Fan Pin-Zhong and Xu Zhi-Zhan
Institution:State Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China
Abstract:We propose a scheme to generate isolated attosecond pulses in the water-window spectral region. Based on the numerical solutions of the single active electron model, we investigate high-order harmonic generation in helium atoms driven by a multi-cycle two-colour optical field synthesized by an intense 2000 nm, 20 fs pulse and its frequency-doubled pulse. When the latter is slightly detuned and properly phase shifted with respect to the fundamental laser pulse, an ultra-broad extreme ultraviolet supercontinuum with a spectral width of 130~eV can be generated in the 270--400~eV spectral regions. A supercontinuum from 280--340~eV in the water window can be selected to yield an isolated 67 attosecond pulse without employing any phase compensation. This water window coherent x-ray pulse with less than 100 attosecond duration is a potential tool for studying the ultrafast electronic dynamics of biological samples in water.
Keywords:x-ray  ultraviolet spectra  optical harmonic generation
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