Continuous wave and tunable laser operation of Yb3+ in disordered NaLa(MoO4)2

Continuous-wave Yb³⁺ laser operation is studied in single crystals of disordered NaLa(MoO₄)₂ at room temperature. The sample used was grown by the Czochralski technique and incorporates an Yb ion density of 3.1×10²⁰ cm^-3. The effect of the Yb concentration on some of the crystal properties is described as well as the spectroscopic Yb³⁺ properties at 5 K. Maximum slope efficiencies of about 40% for π and 38% for σ polarization were obtained under Ti:sapphire laser pumping near 976 nm, respectively. The maximum output power for the π polarization was 400 mW at 1039.5 nm, the threshold in this case amounted to 240 mW (absorbed pump power). The laser emission was tunable between 1016 and 1064 nm with a Lyot filter. Lasing was also realized by pumping with a fiber-coupled diode laser module. Maximum output power of 900 mW at 1035 nm was achieved in this case for the π polarization and the threshold was 280 mW. The results, in terms of output power and tunability, are superior in comparison to all previous reports on Yb-doped disordered double tungstate or molybdate crystals and represent a significant improvement in comparison to earlier experiments with low-doped Yb:NaLa(MoO₄)₂.PACS 42.55.Rz; 42.55.Xi; 42.70.Hj