Influence of Bonner sphere response functions above 20 MeV on unfolded neutron spectra and doses

Monte Carlo (MC) codes for neutron transport calculations such as MCNP, MCNPX, FLUKA, PHITS, and GEANT4, crucially rely on cross sections that describe the interaction of neutrons with nuclei. For neutron energies below 20 MeV, evaluated cross sections are available that are validated against experimental data. In contrast, for high energies (above 20 MeV) experimental data are scarce and, for this reason, every neutron transport code is based on theoretical nuclear models to describe interactions of neutrons with nuclei in matter. Here we report on the calculation of a complete set of response functions for a Bonner spheres spectrometer (BSS), by means of GEANT4 using the Bertini and Binary Intranuclear Cascade (INC) models for energies above 20 MeV. The recent results were compared with those calculated by MCNP/LAHET and MCNP/HADRON MC codes. It turns out that, whatever code used, the response functions were rather similar for neutron energies below 20 MeV, for all 16 detector/moderator combinations of the considered BSS system. For higher energies, however, differences of more than a factor of 2 were observed, depending on neutron energy, detector/moderator combination, MC code, and nuclear model used. These differences are discussed in terms of neutron fluence rates measured at the environmental research station (UFS), “Schneefernerhaus”, (Zugspitze mountain, Germany, 2650 m a.s.l.) for energies below 0.4 eV (thermal neutrons), between 0.4 eV and 100 keV (epithermal neutrons), between 100 keV and 20 MeV (evaporation neutrons), and above 20 MeV (cascade neutrons). In terms of total neutron fluence rates, relative differences of up to 4% were obtained when compared to the standard MCNP/LAHET results, while in terms of total ambient dose equivalent, relative differences of up to 8% were obtained. Both the GEANT4 Binary INC and Bertini INC gave somewhat larger fluence and dose rates in the epithermal region. Most relevant for dose, however, those response functions calculated with the GEANT4 Bertini INC model provided about 18% less neutrons in the cascade region, which led to a roughly 13% smaller contribution of these neutrons to ambient dose equivalent. It is concluded that doses from secondary neutrons from cosmic radiation as deduced from BSS measurements are uncertain by about 10%, simply because of some differences in nuclear models used by various neutron transport codes.