无格点基底表面的杂质分布对分枝状凝聚体的影响

根据含杂质熔融玻璃表面金原子凝聚的实验规律，在原子团簇具有随机的线扩散步长和刚性转动角的特征条件下，建立了含杂质无格点基底表面上改进的杂质限制团簇-团簇(IRCCA)凝聚模型.对团簇的扩散、刚性转动以及凝聚全过程进行了计算机模拟，系统地研究了杂质区域分布情况对分枝状凝聚体诸多特性的影响.结果表明规则分布的杂质对凝聚体生长的影响比随机分布的杂质大，导致杂质规则分布的基底表面上的分枝状凝聚体的数密度更大，分枝状凝聚体的回旋半径，凝聚体平均大小及分形维数更小. 关键词： 薄膜生长 Monte Carlo模拟 分形 杂质

Distribution of impurities on nonlattice substraes influence for fractal aggregates

According to the experimental observation of Au atomic aggregations on a molten glass surface, we established a computational model to simulate Improved Restricted Cluster-Cluster Aggregation (IRCCA) on nonlattice substrates with regularly and randomly distributed impurities. In the model, the random diffusion step and rigidity rotation around the mass center of cluster were considered. The aggregation process was simulated and the influence of the distribution of impurity on the properties of aggregations was systemically investigated. The results show that regularly distributed impurities play a more important role in restricting the aggregation of clusters than randomly distributed impurities, resulting in a higher number density of fractal aggregates with smaller radius of gyration and fractal dimension.