Ultrafast heat transfer on nanoscale in thin gold films |
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Authors: | K V Poletkin G G Gurzadyan J Shang V Kulish |
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Institution: | (1) Division of Thermal and Fluids Engineering, School of Mechanical & Aerospace Engineering, Nanyang Technological University, 50 Nanyang Ave., Singapore, 639798, Singapore;(2) Division of Physics and Applied Physics, School of Physical & Mathematical Sciences, Nanyang Technological University, 21 Nanyang Link, Singapore, 637371, Singapore; |
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Abstract: | Heat transfer processes, induced by ultrashort laser pulses in thin gold films, were studied with a time resolution of 50
fs. It is demonstrated that in thin gold films heat is transmitted by means of electron–phonon and phonon–phonon interactions,
and dissipated on nanoscale within 800 fs. Measurements show that the electron–phonon relaxation time varies versus the probe
wavelength from 1.6 to 0.8 ps for λ=560–630 nm. The applied mathematical model is a result of transforming the two-temperature model to the hyperbolic heat equation,
based on assumptions that the electron gas is heated up instantaneously and applying Cattaneo’s law to the phonon subsystem,
agrees well with the experimental results. This model allows us to define time of electron–phonon scattering as the ratio
of the heat penetration depth to the speed of sound in the bulk material that, in turn, provides an explanation of experimental
results that show the dependence of the electron–phonon relaxation time on the wavelength. |
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