Enhanced ferroelectric,piezoelectric and dielectric properties of (1-x)CaBi2Nb2O9-xBaZr0.2Ti0.8O3 high-temperature piezoelectric composite ceramics |
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Affiliation: | 1. Key Laboratory of Materials Physics, Institute of Solid State Physics, Chinese Academy of Sciences, Hefei, 230031, People''s Republic of China;2. University of Science and Technology of China, Hefei, 230026, People''s Republic of China;3. High Magnetic Field Laboratory, Chinese Academy of Sciences, Hefei, 230031, People''s Republic of China;4. Collaborative Innovation Center of Advanced Microstructures, Nanjing University, Nanjing, 210093, People''s Republic of China |
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Abstract: | Among Aurivillius layer-structured materials, CaBi2Nb2O9 is a best potential candidate for ultrahigh-temperature applications because of its highest Curie temperature of about 940 °C. In this paper, (1-x)CaBi2Nb2O9-xBaZr0.2Ti0.8O3 composite ceramics were prepared by conventional solid-state sintering method. The dielectric results show that the introduction of BaZr0.2Ti0.8O3 not only increases the permittivity of the material, but also reduces its dielectric loss. The optimum electrical properties were obtained in the x = 0.01 sample with piezoelectric coefficient (d33) of 15.1 pC/N and high ferroelectric remnant polarization (Pr) of 9.9 μC/cm2. Furthermore, the composite samples show good thermal depoling performance, the d33 of the x = 0.01 sample is 13.8 pC/N, which is about 91% of the initial value after depoling at 800 °C. Therefore, (1-x)CaBi2Nb2O9-xBaZr0.2Ti0.8O3 is one of the candidates for high temperature piezoelectric materials. |
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Keywords: | Piezoelectricity Dielectric High temperature |
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