Synthesis of phosphonic acid silver-graphene oxide nanomaterials with photocatalytic activity through ultrasonic-assisted method |
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Institution: | 1. College of Chemistry and Material Science, Hebei Normal University, Shijiazhuang 050024, PR China;2. College of Huihua, Hebei Normal University, Hebei, Shijiazhuang 050024, PR China;3. The Real Estate CO., Ltd. of CSCEC, Beijing 100070, PR China |
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Abstract: | In this article, phosphonic acid silver-graphene oxide nanomaterials (Nano-PAS-GO) was synthesized from silver nitrate (AgNO3) solution and phosphoric graphene oxide (PGO) via the convenient ultrasonic-assisted method, and the structure and morphology were characterized, and the photocatalytic activity and recyclability were evaluated through photocatalyzing degradation of Rhodamin B (RhB) aqueous solution, and the possible photocatalytic mechanism was also discussed. Based on those, it was confirmed that Nano-PAS-GO has been synthesized from AgNO3 solution and PGO colloidal suspension under ultrasonic-assisted condition, and Nano-PAS-GO has consisted of phosphoric acid silver nanoparticles and GO with 2D lattice (2D GO lattice) connected in the form of C-P bonds, and the photodegradation rate of Nano-PAS-GO for RhB aqueous solution has reached 93.99%, and Nano-PAS-GO has possessed the nicer recyclability when the photocatalytic time was 50 min. From those results, the strong and stable interface .between PAS nanoparticles and 2D GO lattice connected in the form of the covalent bonds has effectively inhibited the occurrence of the photocorrosion phenomenon. |
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Keywords: | Phosphonic acid silver-graphene oxide nanomaterials (Nano-PAS-GO) Ultrasonic assistance Interface connection Photocatalytic activity Recyclability |
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