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Nonadiabatic electronic response in atom scattering from metal surfaces
Affiliation:1. Max-Planck-Institut für Kohlenforschung, 45470 Mülheim an der Ruhr, Germany;2. Aix Marseille Univ, CNRS, ICR, Marseille, France;1. Key Laboratory of Biobased Materials, Qingdao Institute of Bioenergy and Bioprocess Technology, Chinese Academy of Sciences, Qingdao 266101, Shandong, People’s Republic of China;2. University of Chinese Academy of Sciences, Beijing 100049, People’s Republic of China;3. School of Science, Department of Chemistry, Xi’an Jiaotong University, Xi’an 710049, People’s Republic of China;4. Key Laboratory of Theoretical and Computational Photochemistry, Ministry of Education, College of Chemistry, Beijing Normal University, Beijing 100875, People’s Republic of China;1. State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics (DICP), Chinese Academy of Sciences, 457 Zhongshan Road, Dalian, Liaoning, 116023, China;2. University of Chinese Academy of Sciences, Beijing, 10049, China;1. Los Alamos National Laboratory, Los Alamos, NM 87545, USA;2. Skolkovo Institute of Science and Technology, Moscow 143026, Russia;3. Universidad Nacional de Quilmes, Roque Saenz Pea 352, B1876BXD Bernal, Argentina;1. Center for Computational Sciences, University of Tsukuba, Tennodai 1-1-1, Tsukuba 305-8577, Japan;2. Graduate School of Natural Science and Technology, Faculty of Science, Okayama University, Okayama 700-8530, Japan;3. Riken Advanced Institute for Computational Science, Kobe, Hyogo 650-0047, Japan;4. Institute for NanoScience Design, Osaka University, Toyonaka, Osaka 560-8531, Japan;5. Handairigaku Techno-Research (NPO), Toyonaka, Osaka 560-0043, Japan
Abstract:The response of metal electrons to a localized perturbation varying in time is singular; this dynamic property may influence the observability of diffraction peaks in atom scattering from metal surfaces.
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