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An easily accessible Re-based catalyst for the selective conversion of methanol: evidence for an unprecedented active site structure through combined operando techniques |
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| Authors: | Yoboué Anthony Susset Audrey Tougerti Asma Gallego Daniel Ramani Sudarsan Venkat Kalyanikar Malathi Dolzhnikov Dmitriy S Wubshet Sileshi G Wang Yilun Cristol Sylvain Briois Valérie La Fontaine Camille Gauvin Régis M Paul Jean-François Berrier Elise |
| Affiliation: | Université Lille-Nord de France, 59000 Lille, France. |
| Abstract: | Heterogeneous Re/SiO(2) catalysts prepared using a one pot sol-gel synthesis were found to display high activity in the direct, selective methanol conversion to methylal, which is correlated to an unprecedented rhenium oxide structure. |
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