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Generation of large fifth-order nonlinear phase shifts by use of lossless χ~((2)) cascaded nonlinear processes
作者姓名:XU Guang  QIAN Liejia  WANG Tao  FAN Dianyuan  & LI Fuming . Shanghai Institute of Optics and Fine Mechanics  Chinese Academy of Sciences  Shanghai  China  . State Key Laboratory for Advanced Photonic Materials and Devices  Fudan University  Shanghai  China Correspondence should be addressed to Xu Guang
摘    要:Theinherentthird-ordernonlinearityofmaterialc(3)isnormallyweak.Toaccumulatealargenonlinearphaseshift,highlaserintensityandlongopticalpathinmaterialareneeded.Whilethevalueofnonlinearitycouldbemadelargerneartheregionofabsorptionresonance,astronglosswillbeaccompaniedthroughtheprocessoftwo-photonabsorption.Inordertorealizestrongthird-ordernonlinearitywithcontrollableenergyloss,thec(2)(w;2w,-w)︰c(2)(2w;w,w)cascadingprocesshasbeenproposed,whichisequivalenttothethird-ordernonlinearityc(3)(w;w,w,-w)w…

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