| Recent Progress in Direct Partial Oxidation of Methane to Methanol |
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| 作者姓名： | QijianZhang DehuaHe QimingZhu |
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| 作者单位： | [1]StateKeyLaboratoryofC1ChemistryandTechnology,DepartmentofChemistry,TsinghuaUniversity,Beijing100084,China;LiaoningInstituteofTechnology,Jinzhou121001,China [2]StateKeyLaboratoryofC1ChemistryandTechnology,DepartmentofChemistry,TsinghuaUniversity,Beijing100084,China |
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| 摘 要： | The direct conversion of methane to methanol has attracted a great deal of attention for nearly a century since it was first found possible in 1902, and it is still a challenging task. This review article describes recent advancements in the direct partial oxidation of methane to methanol. The history of direct oxidation of methane and the difficulties encountered in the partial oxidation of methane to methanol are briefly summarized. Recently reported developments in gas-phase homogeneous oxidation, heterogeneous catalytic oxidation and liquid phase homogeneous catalytic oxidation of methane axe reviewed.
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| 关 键 词： | 甲烷 甲醇 氧化处理 气相均匀氧化 液相 催化剂 天然气 |
Recent Progress in Direct Partial Oxidation ofMethane to Methanol |
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| QijianZhang DehuaHe QimingZhu.Recent Progress in Direct Partial Oxidation of Methane to Methanol[J].Journal of Natural Gas Chemistry,2003,12(2):81-89. |
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| Authors: | Qijian Zhang Dehua He Qiming Zhu |
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| Institution: | State Key Laboratory of C1 Chemistry and Technology, Department of Chemistry, Tsinghua University, Beijing 100084, China; 2 Liaoning Institute of Technology, Jinzhou 121001, China |
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| Abstract: | The direct conversion of methane to methanol has attracted a great deal of attention for nearly a century since it was first found possible in 1902, and it is still a challenging task. This review article describes recent advancements in the direct partial oxidation of methane to methanol. The history of direct oxidation of methane and the difficulties encountered in the partial oxidation of methane to methanol are briefly summarized. Recently reported developments in gas-phase homogeneous oxidation, heterogeneous catalytic oxidation and liquid phase homogeneous catalytic oxidation of methane are reviewed. |
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| Keywords: | methane methanol catalytic partial oxidation gas-phase homogeneous oxidation catalyst |
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