A facile construction of the tricyclic 5-7-6 scaffold of fungi-derived diterpenoids. The first total synthesis of (±)-heptemerone G and a new approach to Danishefsky’s intermediate for a guanacastepene A synthesis期刊界 All Journals 搜尽天下杂志传播学术成果专业期刊搜索期刊信息化学术搜索

A facile construction of the tricyclic 5-7-6 scaffold of fungi-derived diterpenoids. The first total synthesis of (±)-heptemerone G and a new approach to Danishefsky’s intermediate for a guanacastepene A synthesis

Authors:	Karol Michalak

Affiliation:	Institute of Organic Chemistry, Polish Academy of Sciences, ul. Kasprzaka 44/52, 01-224 Warsaw 42, Poland

Abstract:	The first total synthesis of (±)-heptemerone G, a diterpenoid metabolite of a submerged culture Coprinus heptemerus, and a new approach to an advanced intermediate for a synthesis of guanacastepene A are reported.

Keywords:	Annulation reactions Medium-ring compounds Quaternary stereocenters Terpenoids Total synthesis
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