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Spin dynamics investigated by EPR in the paramagnetic regime of La2/3Ca1/3Mn1−x Me x O3 (Me = Al, In) manganites
Authors:L. V. Giurgiu  M. N. Grecu  X. Filip  O. Raita  Al. Darabont  D. Gavre  J. Blasco
Affiliation:1. National Institute for Research and Development of Isotopic and Molecular Technologies, P.O. Box 700, 3400, Cluj-Napoca, Romania
2. National Institute for Material Physics, Bucharest, Romania
3. Faculty of Physics, Babes-Bolyai University, Cluj-Napoca, Romania
4. Departmento de Fisica de la Materia Condensada, Universidad de Zaragoza, Zaragoza, Spain
Abstract:
We report an electron paramagnetic resonance (EPR) investigation of the spin dynamics in the paramagnetic regime of the colossal magnetoresistive manganites La2/3Ca1/3Mn1?x Me x O3 (Me=Al, In;x≤0.05). The temperature dependences of the EPR linewidth and integral intensity have been analyzed in terms of the bottleneck spin relaxation and small-polaron hopping models. The exchange coupling integral between Mn3+ and Mn4+ ions and the polaron activation energy decrease with increasing doping level. A discussion is given concerning the factors which could explain the observed changes.
Keywords:
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