Department of Pure and Applied Sciences, College of General Education, University of Tokyo, Komaba, Meguro-ku, Tokyo 153, Japan
Abstract:
The v3 mode of CH3F was excited by irradiation with a TEA CO2 laser pulse, and the time-resolved emission spectra of the v3 overtone and the 3 μ;m region were observed. The results indicate that the population of the v4 level behaves kinetically in the same manner as that of 2v3 or 3v3. This suggests an efficient energy transfer between these levels.