Thermodynamics of crystalline nanonucleus formation from liquid phase |
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Authors: | B I Kidyarov |
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Institution: | 1.Institute of Semiconductor Physics, Siberian Branch,Russian Academy of Sciences,Novosibirsk |
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Abstract: | The energy of crystal nucleation from liquid phase was considered, with the following two stages taken into account: (1) the formation of metastable supercooled melt (solution), containing pre-nuclei with intermediate amorphous (quasicrystalline) structure, and (2) the transformation of amorphous clusters into solid crystalline nuclei having different structures. With growth of a nucleus the nucleation energy profile manifests 2–3 maxima corresponding to these stages, and the kinetics of the non-stationary nucleation has five characteristic variations. |
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