Noncollinear second harmonic generation in KDP

This paper reports experimental and analytical results on optical second harmonic generation when a noncollinear arrangement is employed. The dependence of second harmonic power on crystal length, absorption, beam radius and the angle between the two fundamental waves is obtained. Double refraction of the crystal is taken into account, but the divergence and depletion of the fundamental waves are neglected. The results of the calculations are confirmed by experiments carried out with a KDP crystal in the near field of two intersecting TEM₀₀ ruby laser beams.An extension of the theory to nonlinear interactions other than second harmonic generation - e.g. four-wave interaction - is possible.