薄原子蒸汽膜的双光子光谱及Dicke窄化

薄原子蒸汽膜的单光子Dcike窄化吸收光谱可以拓展到双光子情形，以级联三能级系统为例,从理论上得到了亚多普勒结构的双光子吸收光谱，其线型表现出和单光子过程相似的与膜厚和探测光波长的比值(L/λ)相关的周期性.当L/λ=(2n+1)/2(膜厚为半波长的奇数倍)时，吸收谱线窄化现象明显.当L/λ=2n/2(膜厚为半波长的偶数倍)时，单光子情形的谱线窄化现象消失，而双光子情形的谱线仍表现为亚多普勒结构，尤其在异侧入射的情形下，可以获得极窄的双光子谱线结构. 这种结构来自原子与腔壁碰撞的消激发效应和双光子过程的抽运-探测机制的贡献. 关键词： 薄原子蒸汽膜 双光子光谱 Dicke窄化

Two-photon spectroscopy and Dicke narrowing of a thin atomic vapor film

One-photon Dick-narrowing absorption spectroscopy from a thin atomic vapor film can be extended to the two-photon case, in which the sub-Doppler absorption structures are obtained in a cascade three-level system. The periodic line shapes of two photon spectroscopy are similar to one-photon case. It is found that Dicke-narrowing is apparent when L/λ=(2n+1)/2 (n an integer, L the film thickness, and λ the wavelength of the probe field)in the case of one-photon process, and this feature is maintained in the case of two-photon process but not in the one-photon process when L/λ=2n/2. Due to the contribution of atom-wall collision in the cell and the pump-probe scheme, a very narrow structure can be obtained when the pump and the probe fields are in counter-propagation regime.