Abstract: | Fe3O4@SiO2‐Ag catalyst was found to be highly active and selective in the N ‐alkylation of amines with a variety of aromatic and linear alcohols. The heterogeneous nature of the Fe3O4@SiO2‐Ag catalyst allows easy recovery and regeneration by applying an external magnet for six subsequent reaction cycles. The prepared catalyst was characterized using electron microscopy techniques, X‐ray diffraction, vibrating sample magnetometry and atomic absorption spectroscopy. |