Laboratory intercomparison of the ozone absorption coefficients in the mid-infrared (10 microm) and ultraviolet (300-350 nm) spectral regions |
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Authors: | Picquet-Varrault B Orphal J Doussin J-F Carlier P Flaud J-M |
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Institution: | Laboratoire Interuniversitaire des Systèmes Atmosphériques, UMR-CNRS 7583, University of Paris 7 and Paris 12, 94010 Créteil cedex, France. picquet@lisa.univ-paris12.fr |
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Abstract: | For the measurement of atmospheric ozone concentrations, the mid-infrared and ultraviolet regions are both used by ground-, air-, or satellite-borne instruments. In this study we report the first laboratory intercomparison of the ozone absorption coefficients using simultaneous measurements in these spectral regions. The intercomparison shows good agreement (around 98.5%) between the HITRAN 2000 recommendation for the mid-infrared and the most reference measurements in the ultraviolet regions, whereas systematic differences of about 5.5% are observed when using the recommendation of HITRAN2003 for the mid-infrared. Possible reasons for this discrepancy are discussed. Future measurements are clearly needed to resolve this issue. |
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