Critical energy for direct initiation of detonation induced by laser ablation

This study describes experimental work examining the critical energy for direct initiation of detonation by laser ablation in a stoichiometric acetylene–oxygen mixture. The amount of input energy, the target material, and the surface roughness of the target were varied to study their effects on shock wave generation. Aluminum and stainless steel were used as target materials. The propagating shock wave induced by laser ablation was observed using high-speed shadow imaging. The critical energy for direct initiation of detonation was calculated using the strong blast wave theory. The critical input energy for aluminum was found to be lower than that for stainless steel. Because the thermodynamic critical temperature of aluminum is lower than that of stainless steel, aluminum caused a phase explosion more easily than stainless steel, thus resulting in direct initiation of detonation with a lower amount of input energy. The effects of surface roughness on critical input energy and shock wave generation were negligibly small. The critical initiation energy was estimated to be \(10.3 \pm 0.2\) mJ, which is in agreement with the experimental data obtained in previous work. The estimated critical initiation energy was independent of the target material. However, other predictions of the critical initiation energy by using the cell size overestimated this value because of the scatter in cell size data of an unstable cellular structure. Furthermore, interaction between plasma plumes formed by laser ablation and those formed by breakdown near the target surface might have contributed to requiring a lower amount of energy for initiating detonation.