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Mass distribution in the bremsstrahlung-induced fission of Th,U and Pu
Authors:H Naik  VT Nimje  D Raj  SV Suryanarayana  A Goswami  Sarbjit Singh  SN Acharya  KC Mittal  S Ganesan  P Chandrachoodan  VK Manchanda  V Venugopal  S Banarjee
Institution:1. Radiochemistry Division, Bhabha Atomic Research Centre, Mumbai, 400085, India;2. Accelerator and Pulse Power Division, BARC, Mumbai, 400085, India;3. Reactor Physics Design Division, BARC, Mumbai, 400085, India;4. Nuclear Physics Division, BARC, Mumbai, 400085, India;5. Board of Research in Nuclear Science, BARC, Mumbai, 400085, India;6. Chairman, Atomic Energy Commission, Mumbai, 400085, India
Abstract:The yields of various fission products in the 10 MeV bremsstrahlung-induced fission of 232Th, 238U and 240Pu were determined using a recoil catcher and off-line γ-ray spectrometric techniques. From the yield data, mass yield distributions were obtained using charge distribution corrections. The higher yields of fission products around mass numbers 133–135, 138–140, 143–145 and their complementary products in the neutron and bremsstrahlung-induced fission of 232Th, 238U and 240Pu were interpreted based on nuclear structure effects. From the mass yield distribution, the peak-to-valley (P/VP/V) ratio was also obtained for the above fissioning systems. The present data, along with data from the literature on different bremsstrahlung- and mono-energetic neutron-induced fissions of 232Th and 238U are interpreted to examine the influence of excitation energy on the peak to valley ratio. For the same compound nucleus 240Pu?, the data in the 10–30 MeV bremsstrahlung-induced fission of 240Pu were compared with similar data of thermal to 14 MeV neutron-induced fission of 239Pu and the spontaneous fission of 240Pu to examine the role of excitation energy due to bremsstrahlung radiation and mono-energetic neutrons.
Keywords:Nuclear reactions  +232Th  +238U  +240Pu(γ  F)  E=10   MeVE=10 " target="_blank">gif" overflow="scroll">E=10   MeV bremsstrahlung  measured fission yields and mass distributions via off-line γ-spectroscopy using an HPGe detector  Comparison with neutron-induced fission data
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