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Thermal and chemical nanofractal relaxation
Authors:C Bréchignac  Ph Cahuzac  F Carlier  C Colliex  M de Frutos  N Kébaïli  J Le Roux  A Masson and B Yoon
Institution:(1) Laboratoire Aimé Cotton, CNRS, bâtiment 505, Université Paris-Sud, 91405 Orsay Cedex, France;(2) Laboratoire de Physique des solides, bâtiment 510, Université Paris-Sud, 91405 Orsay Cedex, France
Abstract:We studied shape relaxation of nano-fractal islands, during annealing, after their growth from antimony cluster deposition on graphite surface. Annealing at 180°C shows evidence of an increase of the fractal branch width with time followed by branch fragmentation, without changing the fractal dimension. The time evolution of the width of the arm suggests the surface self-diffusion mechanism as the main relaxation process. With Monte Carlo simulations, we confirmed the observed behavior. Comparison is done with our previous results on fragmentation of nano-fractal silver islands when impurity added to the incident cluster promotes rapid fragmentation by surface self-diffusion enhancement 1].
Keywords:61  46  +w Nanoscale materials: clusters  nanoparticles  nanotubes  and nanocrystals  61  43  Hv Fractals  macroscopic aggregates (including diffusion-limited aggregates)  81  07  -b Nanoscale materials and structures: fabrication and characterization
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