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Engineering Graphdiyne for Solar Photocatalysis |
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| Authors: | Dr. Jian Li Lei Zhu Prof. Dr. Chen-Ho Tung Prof. Dr. Li-Zhu Wu |
| Affiliation: | 1. Key Laboratory of Photochemical Conversion and Optoelectronic Materials, Technical Institute of Physics and Chemistry & University of Chinese Academy of Sciences, Chinese Academy of Sciences, Beijing, 100190 P. R. China;2. Key Laboratory of Photochemical Conversion and Optoelectronic Materials, Technical Institute of Physics and Chemistry & University of Chinese Academy of Sciences, Chinese Academy of Sciences, Beijing, 100190 P. R. China New Cornerstone Science Laboratory, Shenzhen, 518054 P. R. China |
| Abstract: | Graphdiyne (GDY) with a direct band gap, excellent carrier mobility and uniform pores, is regarded as a promising photocatalytic material for solar energy conversion, while the research on GDY in photocatalysis is a less developed field. Herein, the distinctive structure, adjustable band gap, and electronic properties of GDY for photocatalysis is firstly summarized. The construction and progress of GDY-based photocatalysts for solar energy conversion, including H2 evolution reaction (HER), CO2 reduction reaction (CO2RR) and N2 reduction reaction (NRR) are then elaborated. At last, the challenges and perspectives in developing GDY-based photocatalysts for solar fuel production are discussed. It is anticipated that a timely Minireview will be helpful for rapid progress of GDY in solar energy conversion. |
| Keywords: | CO2 Reduction Graphdiyne H2 Evolution Heterojunctions Photocatalysis |