One-pot synthesis of core-expanded naphthalene diimides: enabling N-substituent modulation for diverse n-type organic materials |
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| Authors: | Hu Yunbin Qin Yunke Gao Xike Zhang Fengjiao Di Chong-an Zhao Zheng Li Hongxiang Zhu Daoben |
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| Affiliation: | Laboratory of Materials Science, Shanghai Institute of Organic Chemistry, Chinese Academy of Sciences (CAS), 345 Lingling Road, Shanghai 200032, China. |
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| Abstract: | A mild and versatile one-pot synthesis of core-expanded naphthalene diimides has been developed, which undergoes a nucleophilic aromatic substitution reaction and then an imidization reaction, allowing an easy and low-cost access to diverse n-type organic materials. Some newly synthesized compounds by this one-pot operation exhibited high electron mobility of up to 0.70 cm(2) V(-1) s(-1) in ambient conditions. |
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