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Fluctuating Electric Field Gradients at 111Cd in Ice
Authors:Akselrod  Z. Z.  Filossofov  D. V.  Kochetov  O. I.  Korolev  N. A.  Lebedev  N. A.  Milanov  M.  Novgorodov  A. F.  Shirani  E. N.  Timkin  V. V.  Velichkov  A. I.
Affiliation:(1) Skobeltsyn Institute of Nuclear Physics, Moscow State University, 119899 Moscow, Russia;(2) Joint Institute for Nuclear Research, LNP, P.O. Box 79, Moscow, Russia;(3) Institute for Nuclear Research, BAS, 1000 Sofia, Bulgaria;(4) Vereshchagin Institute of High Pressure Physics, RAS, 142092 Troitsk, Moscow reg., Russia
Abstract:111Cd–PAC measurements have been made using the high specific activity of 111In in the methanol–water mixtures of various concentrations at the room temperature. These experiments revealed that the perturbation factors 〈A 2 G 2〉 (integrated over two mean lives τN) do not follow the dependence of the macroscopic viscosity η. The observed dynamic character of the PAC spectra in ice is explained by the mobility of orientational and ionic defects. The activation energy for the diffusion process was determined to be E a =0.35(1) eV. This revised version was published online in September 2006 with corrections to the Cover Date.
Keywords:111In   111Cd  high specific activity  nuclear quadrupole interactions (NQI)  TDPAC
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