Enhanced Photocatalytic H2-production Activity of CdS Nanoflower using Single Atom Pt and Graphene Quantum Dot as Dual Cocatalysts |
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作者姓名: | Yi Yang Jinsong Wu Bei Cheng Liuyang Zhang Ahmed Abdullah Al-Ghamdi Swelm Wageh Youji Li |
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作者单位: | 1. State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, Nanostructure Research Centre (NRC), Wuhan University of Technology;2. Laboratory of Solar Fuel, Faculty of Materials Science and Chemistry, China University of Geosciences;3. Department of Physics, Faculty of Science, King Abdulaziz University;4. College of Chemistry and Chemical Engineering, Jishou University |
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基金项目: | supported by the National Key Research and Development Program of China (2018YFB1502001);;National Natural Science Foundation of China (NSFC) (Nos. 51872220, 51961135303, 51932007, U1905215, 21871217 and 52073223); |
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摘 要: | Single-atom catalysts have high catalytic activity due to their unique quantum size effects and optimal atom utilization. Herein, visiblelight-responsive photocatalysts were designed by coupling Cd S with graphene quantum dots(GQDs) and platinum single atoms(Pt SAs). GQDs and Pt SAs were successively loaded on ultrathin Cd S nanosheets through freeze-drying and in-situ photocatalytic reduction. The synergistic effect between Pt SAs and GQDs results in superior photocatalytic activity with a hydr...
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