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Coherent phonon dynamics of normal metal in ultrafast spectroscopy: Non-equilibrium gauge invariant Green's function approach
Affiliation:1. Department of Solid State Physics, Yerevan State University, Alex Manoogian 1, 0025 Yerevan, Armenia;2. National University of Architecture and Construction of Armenia, Teryan 105, 0009 Yerevan, Armenia;3. Instituto de Alta Investigación, Universidad de Tarapacá, Casilla 7D, Arica, Chile;4. SUPA School of Physics and Astronomy, University of Glasgow, Glasgow G12 8QQ, United Kingdom;1. Department of Applied Physics, University for Development Studies, Navrongo, Ghana;2. Department of Physics, College of Agriculture and Natural Sciences, U.C.C., Ghana;3. Department of Mathematics, College of Agriculture and Natural Sciences, U.C.C., Ghana;1. Department of Physics and Engineering, Moldova State University, Chisinau MD-2009, Republic of Moldova;2. Institute of Applied Physics, Moldavian Academy of Science, Chisinau MD-2028, Republic of Moldova;3. Gwangju Institute of Science and Technology, Gwangju 500-712, Republic of Korea;1. Department of Physics and Astronomy, University of Manitoba, Winnipeg, Canada R3T 2N2;2. Department of Physics/Theoretical Physics, University of Oulu, Oulu FIN-90014, Finland;1. School of Materials Science and Engineering, Shandong Jianzhu University, Fengming Road #1000, Jinan 250101, PR China;2. Department of Chemical and Materials Engineering, University of Kentucky, Lexington, KY 40506, USA;3. Beijing Aeronautical Manufacturing Technology Research Institute, Beijing 100024, PR China
Abstract:
The phonon dynamics of normal metal in the coherent regime of ultrafast spectroscopy is studied based on the non-equilibrium gauge invariant Green's function method. The non-equilibrium phonon self-energy is computed explicitly as a function of time in a gauge invariant way up to the second order of electric field of applied laser pulse. The extension beyond the coherent regime and the incorporation of correlation effects are discussed.
Keywords:Ultrafast spectroscopy  Quantum Boltzmann equation  Gauge invariance  Phase coherent dynamics  Phonon dynamics
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