μ+SR frequency shifts in the van‐Vleck paramagnet PrIn3

As part of an ongoing μ⁺SR study on cubic van‐Vleck paramagnets of the PrM₃ series ( M\ =\ In,Pb,Tl,Sn), in which the CEF level scheme varies systematically, we present preliminary static μ⁺SR results on a single crystal of PrIn₃. From the angular dependence and from the appearance of the μSR spectra, we could determine that stopped μ⁺ occupy octahedral sites of the (1/2, 0, 0) type, i.e. sites with 2 Pr and 4 In atoms as neighbors. The spectral frequency shifts can be accounted for by assigning to the Pr sites essentially unperturbed 4f dipole moment values, as derived from bulk magnetization measurements. The temperature dependence of the shifts scales to a good accuracy with the bulk susceptibility. It is concluded that unlike previous observations with PrNi₅, the local perturbations induced by an interstitial μ⁺ on the CEF levels of neighboring Pr in the PrIn₃ system are small compared with the unperturbed level splitting itself. This revised version was published online in July 2006 with corrections to the Cover Date.