On the Lowest Energy Nucleation Path in a Supersaturated Lattice Gas |
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Authors: | Vitaly A. Shneidman |
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Affiliation: | (1) Department of Physics, New Jersey Institute of Technology, Newark, New Jersey, 07102 |
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Abstract: | A lattice gas with non-conserved spin flip dynamics (of both non-Glauber and Glauber types) is considered at TTc, the critical temperature. For arbitrary supersaturation, S, a general expression for the inverse of the nucleation rate along the lowest energy path is derived. The exponential part is identical to the one by Neves and Schonmann [Commun. Math. Phys.137:20 (1991)]. The preexponential can be expressed in terms of elliptic theta-functions for small S, and in the limits, respectively, of ST/ or ST/ (– being the nearest-neighbor interaction energy), elementary versions of the general expression are further obtained. The preexponential has a smooth component, as well as small-scale modulations which are approximately periodic in the inverse supersaturation. For ST/, the smooth part is proportional to , in contrast to the zero-T limit where it is linear in S. The latter limit becomes apparent only at extremely low temperatures which are cubic in S. |
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Keywords: | nucleation lattice gas Glauber dynamics preexponential |
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