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Direct alpha spectrometry for characterising hot particle properties
Authors:R. P  ll  nen, T. Siiskonen, M. Moring,J. Juhanoja
Affiliation:

aSTUK - Radiation and Nuclear Safety Authority, P.O. Box 14, FIN-00881 Helsinki, Finland

bTop Analytica Ltd., Ruukinkatu 4, FIN-20540 Turku, Finland

Abstract:
Non-destructive analysis methods, especially direct alpha spectrometry but also gamma ray spectrometry and scanning electron microscopy were applied to a nuclear bomb particle from the Thule accident. The use of high-resolution direct alpha spectrometry with the aid of Monte Carlo simulations was demonstrated here in order to determine the properties of this particle. In general, the information that can be obtained through direct alpha spectrometry depends on the information available a priori. For example, known elemental composition makes the assessment of particle dimensions possible even if scanning electron microscopy images are unavailable. Although direct alpha spectrometry may be applied for particle characterisation, further developments in spectrum analysis tools are necessary.
Keywords:Hot particle   Direct alpha spectrometry   Plutonium   Americium   Thule accident
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