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Dependence of resonance energy transfer on exciton dimensionality
Authors:Rindermann Jan Junis  Pozina Galia  Monemar Bo  Hultman Lars  Amano Hiroshi  Lagoudakis Pavlos G
Affiliation:School of Physics and Astronomy, University of Southampton, Southampton SO17 1BJ, United Kingdom.
Abstract:We investigate the dependence of resonance energy transfer from Wannier-Mott excitons to an organic overlayer on exciton dimensionality. We exploit the excitonic potential disorder in a single quantum well to tune the balance between localized and free excitons by scaling the Boltzmann distribution of excitons through temperature. Theoretical calculations predict the experimentally observed temperature dependence of resonance energy transfer and allow us to quantify the contribution of localized and free excitons. We show that free excitons can undergo resonance energy transfer with an order of magnitude higher rate compared to localized excitons, emphasizing the potential of hybrid optoelectronic devices utilizing resonance energy transfer as a means to overcome charge transfer related limitations.
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